IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-36313-6.html
   My bibliography  Save this article

Realizing nearly-zero dark current and ultrahigh signal-to-noise ratio perovskite X-ray detector and image array by dark-current-shunting strategy

Author

Listed:
  • Peng Jin

    (Zhejiang University)

  • Yingjie Tang

    (Westlake University
    Zhejiang University)

  • Dingwei Li

    (Westlake University
    Zhejiang University)

  • Yan Wang

    (Westlake University
    Zhejiang University)

  • Peng Ran

    (Zhejiang University)

  • Chuanyu Zhou

    (Zhejiang University)

  • Ye Yuan

    (Wuhan University of Technology)

  • Wenjuan Zhu

    (Zhejiang University
    Nanjing University of Posts and Telecommunications)

  • Tianyu Liu

    (Zhejiang University)

  • Kun Liang

    (Westlake University
    Zhejiang University)

  • Cuifang Kuang

    (Zhejiang University
    Intelligent Optics & Photonics Research Center Jiaxing Institute of Zhejiang University)

  • Xu Liu

    (Zhejiang University)

  • Bowen Zhu

    (Westlake University)

  • Yang (Michael) Yang

    (Zhejiang University
    Intelligent Optics & Photonics Research Center Jiaxing Institute of Zhejiang University)

Abstract

Although perovskite X-ray detectors have revealed promising properties, their dark currents are usually hundreds of times larger than the practical requirements. Here, we report a detector architecture with a unique shunting electrode working as a blanking unit to suppress dark current, and it theoretically can be reduced to zero. We experimentally fabricate the dark-current-shunting X-ray detector, which exhibits a record-low dark current of 51.1 fA at 5 V mm−1, a detection limit of 7.84 nGyair s−1, and a sensitivity of 1.3 × 104 μC Gyair−1 cm−2. The signal-to-noise ratio of our polycrystalline perovskite-based detector is even outperforming many previously reported state-of-the-art single crystal-based X-ray detectors by serval orders of magnitude. Finally, the proof-of-concept X-ray imaging of a 64 × 64 pixels dark-current-shunting detector array is successfully demonstrated. This work provides a device strategy to fundamentally reduce dark current and enhance the signal-to-noise ratio of X-ray detectors and photodetectors in general.

Suggested Citation

  • Peng Jin & Yingjie Tang & Dingwei Li & Yan Wang & Peng Ran & Chuanyu Zhou & Ye Yuan & Wenjuan Zhu & Tianyu Liu & Kun Liang & Cuifang Kuang & Xu Liu & Bowen Zhu & Yang (Michael) Yang, 2023. "Realizing nearly-zero dark current and ultrahigh signal-to-noise ratio perovskite X-ray detector and image array by dark-current-shunting strategy," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-36313-6
    DOI: 10.1038/s41467-023-36313-6
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-36313-6
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-023-36313-6?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Jiali Peng & Chelsea Q. Xia & Yalun Xu & Ruiming Li & Lihao Cui & Jack K. Clegg & Laura M. Herz & Michael B. Johnston & Qianqian Lin, 2021. "Crystallization of CsPbBr3 single crystals in water for X-ray detection," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    2. Xiaopeng Zheng & Bo Chen & Jun Dai & Yanjun Fang & Yang Bai & Yuze Lin & Haotong Wei & Xiao Cheng Zeng & Jinsong Huang, 2017. "Defect passivation in hybrid perovskite solar cells using quaternary ammonium halide anions and cations," Nature Energy, Nature, vol. 2(7), pages 1-9, July.
    3. Haotong Wei & Jinsong Huang, 2019. "Halide lead perovskites for ionizing radiation detection," Nature Communications, Nature, vol. 10(1), pages 1-12, December.
    4. Xiangyu Ou & Xian Qin & Bolong Huang & Jie Zan & Qinxia Wu & Zhongzhu Hong & Lili Xie & Hongyu Bian & Zhigao Yi & Xiaofeng Chen & Yiming Wu & Xiaorong Song & Juan Li & Qiushui Chen & Huanghao Yang & X, 2021. "High-resolution X-ray luminescence extension imaging," Nature, Nature, vol. 590(7846), pages 410-415, February.
    5. Yong Churl Kim & Kwang Hee Kim & Dae-Yong Son & Dong-Nyuk Jeong & Ja-Young Seo & Yeong Suk Choi & In Taek Han & Sang Yoon Lee & Nam-Gyu Park, 2017. "Printable organometallic perovskite enables large-area, low-dose X-ray imaging," Nature, Nature, vol. 550(7674), pages 87-91, October.
    6. Yunxia Zhang & Yucheng Liu & Zhuo Xu & Haochen Ye & Zhou Yang & Jiaxue You & Ming Liu & Yihui He & Mercouri G. Kanatzidis & Shengzhong (Frank) Liu, 2020. "Nucleation-controlled growth of superior lead-free perovskite Cs3Bi2I9 single-crystals for high-performance X-ray detection," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Dou Zhao & Ruiling Gao & Wei Cheng & Mengyao Wen & Xinlei Zhang & Tomoyuki Yokota & Paul Sellin & Shengyuan A. Yang & Li Shang & Chongjian Zhou & Takao Someya & Wanqi Jie & Yadong Xu, 2024. "Heavy-to-light electron transition enabling real-time spectra detection of charged particles by a biocompatible semiconductor," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    2. Yingjie Tang & Peng Jin & Yan Wang & Dingwei Li & Yitong Chen & Peng Ran & Wei Fan & Kun Liang & Huihui Ren & Xuehui Xu & Rui Wang & Yang (Michael) Yang & Bowen Zhu, 2023. "Enabling low-drift flexible perovskite photodetectors by electrical modulation for wearable health monitoring and weak light imaging," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    3. Jingxian Zhong & Dawei Zhou & Qi Bai & Chao Liu & Xinlian Fan & Hehe Zhang & Congzhou Li & Ran Jiang & Peiyi Zhao & Jiaxiao Yuan & Xiaojiao Li & Guixiang Zhan & Hongyu Yang & Jing Liu & Xuefen Song & , 2024. "Growth of millimeter-sized 2D metal iodide crystals induced by ion-specific preference at water-air interfaces," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    4. Zihao Song & Xinyuan Du & Xin He & Hanqi Wang & Zhiqiang Liu & Haodi Wu & Hongde Luo & Libo Jin & Ling Xu & Zhiping Zheng & Guangda Niu & Jiang Tang, 2023. "Rheological engineering of perovskite suspension toward high-resolution X-ray flat-panel detector," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Jincong Pang & Haodi Wu & Hao Li & Tong Jin & Jiang Tang & Guangda Niu, 2024. "Reconfigurable perovskite X-ray detector for intelligent imaging," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    2. Robert A. Jagt & Ivona Bravić & Lissa Eyre & Krzysztof Gałkowski & Joanna Borowiec & Kavya Reddy Dudipala & Michał Baranowski & Mateusz Dyksik & Tim W. J. Goor & Theo Kreouzis & Ming Xiao & Adrian Bev, 2023. "Layered BiOI single crystals capable of detecting low dose rates of X-rays," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    3. Yurou Zhang & Miaoqiang Lyu & Tengfei Qiu & Ekyu Han & Il Ku Kim & Min-Cherl Jung & Yun Hau Ng & Jung-Ho Yun & Lianzhou Wang, 2020. "Halide Perovskite Single Crystals: Optoelectronic Applications and Strategical Approaches," Energies, MDPI, vol. 13(16), pages 1-27, August.
    4. Zihao Song & Xinyuan Du & Xin He & Hanqi Wang & Zhiqiang Liu & Haodi Wu & Hongde Luo & Libo Jin & Ling Xu & Zhiping Zheng & Guangda Niu & Jiang Tang, 2023. "Rheological engineering of perovskite suspension toward high-resolution X-ray flat-panel detector," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    5. Nan Gan & Xin Zou & Mengyang Dong & Yanze Wang & Xiao Wang & Anqi Lv & Zhicheng Song & Yuanyuan Zhang & Wenqi Gong & Zhu Zhao & Ziyang Wang & Zixing Zhou & Huili Ma & Xiaowang Liu & Qiushui Chen & Hui, 2022. "Organic phosphorescent scintillation from copolymers by X-ray irradiation," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    6. Lutao Li & Junjie Yao & Juntong Zhu & Yuan Chen & Chen Wang & Zhicheng Zhou & Guoxiang Zhao & Sihan Zhang & Ruonan Wang & Jiating Li & Xiangyi Wang & Zheng Lu & Lingbo Xiao & Qiang Zhang & Guifu Zou, 2023. "Colloid driven low supersaturation crystallization for atomically thin Bismuth halide perovskite," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    7. Yun-Lan Li & Hai-Ling Wang & Zhong-Hong Zhu & Yu-Feng Wang & Fu-Pei Liang & Hua-Hong Zou, 2024. "Aggregation induced emission dynamic chiral europium(III) complexes with excellent circularly polarized luminescence and smart sensors," Nature Communications, Nature, vol. 15(1), pages 1-15, December.
    8. Yanliang Liu & Chaosong Gao & Dong Li & Xin Zhang & Jiongtao Zhu & Meng Wu & Wenjun Liu & Tongyu Shi & Xingchen He & Jiahong Wang & Hao Huang & Zonghai Sheng & Dong Liang & Xue-Feng Yu & Hairong Zheng, 2024. "Dynamic X-ray imaging with screen-printed perovskite CMOS array," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    9. Hailei Zhang & Bo Zhang & Chongyang Cai & Kaiming Zhang & Yu Wang & Yuan Wang & Yanmin Yang & Yonggang Wu & Xinwu Ba & Richard Hoogenboom, 2024. "Water-dispersible X-ray scintillators enabling coating and blending with polymer materials for multiple applications," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    10. Renzhong Zhuang & Songhua Cai & Zengxia Mei & Huili Liang & Ningjiu Zhao & Haoran Mu & Wenzhi Yu & Yan Jiang & Jian Yuan & Shuping Lau & Shiming Deng & Mingyue Han & Peng Jin & Cailin Wang & Guangyu Z, 2023. "Solution-grown BiI/BiI3 van der Waals heterostructures for sensitive X-ray detection," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    11. Yangshuang Bian & Mingliang Zhu & Chengyu Wang & Kai Liu & Wenkang Shi & Zhiheng Zhu & Mingcong Qin & Fan Zhang & Zhiyuan Zhao & Hanlin Wang & Yunqi Liu & Yunlong Guo, 2024. "A detachable interface for stable low-voltage stretchable transistor arrays and high-resolution X-ray imaging," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    12. Xiaopeng Feng & Yuhong He & Wei Qu & Jinmei Song & Wanting Pan & Mingrui Tan & Bai Yang & Haotong Wei, 2022. "Spray-coated perovskite hemispherical photodetector featuring narrow-band and wide-angle imaging," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    13. Da Liu & Yichu Zheng & Xin Yuan Sui & Xue Feng Wu & Can Zou & Yu Peng & Xinyi Liu & Miaoyu Lin & Zhanpeng Wei & Hang Zhou & Ye-Feng Yao & Sheng Dai & Haiyang Yuan & Hua Gui Yang & Shuang Yang & Yu Hou, 2024. "Universal growth of perovskite thin monocrystals from high solute flux for sensitive self-driven X-ray detection," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    14. Liangrui He & Liyang Wang & Xujiang Yu & Yizhang Tang & Zhao Jiang & Guoliang Yang & Zhuang Liu & Wanwan Li, 2024. "Full-course NIR-II imaging-navigated fractionated photodynamic therapy of bladder tumours with X-ray-activated nanotransducers," Nature Communications, Nature, vol. 15(1), pages 1-19, December.
    15. Guus J. W. Aalbers & Tom P. A. Pol & Kunal Datta & Willemijn H. M. Remmerswaal & Martijn M. Wienk & René A. J. Janssen, 2024. "Effect of sub-bandgap defects on radiative and non-radiative open-circuit voltage losses in perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    16. Omar M. Saif & Yasmine Elogail & Tarek M. Abdolkader & Ahmed Shaker & Abdelhalim Zekry & Mohamed Abouelatta & Marwa S. Salem & Mostafa Fedawy, 2023. "Comprehensive Review on Thin Film Homojunction Solar Cells: Technologies, Progress and Challenges," Energies, MDPI, vol. 16(11), pages 1-23, May.
    17. Dou Zhao & Ruiling Gao & Wei Cheng & Mengyao Wen & Xinlei Zhang & Tomoyuki Yokota & Paul Sellin & Shengyuan A. Yang & Li Shang & Chongjian Zhou & Takao Someya & Wanqi Jie & Yadong Xu, 2024. "Heavy-to-light electron transition enabling real-time spectra detection of charged particles by a biocompatible semiconductor," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    18. Rashmi Mehrotra & Dongrak Oh & Ji-Wook Jang, 2021. "Unassisted selective solar hydrogen peroxide production by an oxidised buckypaper-integrated perovskite photocathode," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    19. Yehui Wen & Tianchi Zhang & Xingtao Wang & Tiantian Liu & Yu Wang & Rui Zhang & Miao Kan & Li Wan & Weihua Ning & Yong Wang & Deren Yang, 2024. "Amorphous (lysine)2PbI2 layer enhanced perovskite photovoltaics," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    20. Stefania Cacovich & Guillaume Vidon & Matteo Degani & Marie Legrand & Laxman Gouda & Jean-Baptiste Puel & Yana Vaynzof & Jean-François Guillemoles & Daniel Ory & Giulia Grancini, 2022. "Imaging and quantifying non-radiative losses at 23% efficient inverted perovskite solar cells interfaces," Nature Communications, Nature, vol. 13(1), pages 1-9, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-36313-6. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.