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High field magnetometry with hyperpolarized nuclear spins

Author

Listed:
  • Ozgur Sahin

    (University of California, Berkeley)

  • Erica Leon Sanchez

    (University of California, Berkeley)

  • Sophie Conti

    (University of California, Berkeley)

  • Amala Akkiraju

    (University of California, Berkeley)

  • Paul Reshetikhin

    (University of California, Berkeley)

  • Emanuel Druga

    (University of California, Berkeley)

  • Aakriti Aggarwal

    (University of California, Berkeley)

  • Benjamin Gilbert

    (Lawrence Berkeley National Laboratory)

  • Sunil Bhave

    (Purdue University)

  • Ashok Ajoy

    (University of California, Berkeley
    Lawrence Berkeley National Laboratory)

Abstract

Quantum sensors have attracted broad interest in the quest towards sub-micronscale NMR spectroscopy. Such sensors predominantly operate at low magnetic fields. Instead, however, for high resolution spectroscopy, the high-field regime is naturally advantageous because it allows high absolute chemical shift discrimination. Here we demonstrate a high-field spin magnetometer constructed from an ensemble of hyperpolarized 13C nuclear spins in diamond. They are initialized by Nitrogen Vacancy (NV) centers and protected along a transverse Bloch sphere axis for minute-long periods. When exposed to a time-varying (AC) magnetic field, they undergo secondary precessions that carry an imprint of its frequency and amplitude. For quantum sensing at 7T, we demonstrate detection bandwidth up to 7 kHz, a spectral resolution

Suggested Citation

  • Ozgur Sahin & Erica Leon Sanchez & Sophie Conti & Amala Akkiraju & Paul Reshetikhin & Emanuel Druga & Aakriti Aggarwal & Benjamin Gilbert & Sunil Bhave & Ashok Ajoy, 2022. "High field magnetometry with hyperpolarized nuclear spins," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32907-8
    DOI: 10.1038/s41467-022-32907-8
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    References listed on IDEAS

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