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Comparative Study on the Adsorption Capacities of the Three Black Phosphorus-Based Materials for Methylene Blue in Water

Author

Listed:
  • Juanhong Wang

    (School of Environment, Northeast Normal University, NO. 2555 Jingyue Street, Changchun 130117, China
    These authors contributed equally to this work.)

  • Zhaocheng Zhang

    (School of Environment, Northeast Normal University, NO. 2555 Jingyue Street, Changchun 130117, China
    These authors contributed equally to this work.)

  • Dongyang He

    (School of Environment, Northeast Normal University, NO. 2555 Jingyue Street, Changchun 130117, China)

  • Hao Yang

    (School of Environment, Northeast Normal University, NO. 2555 Jingyue Street, Changchun 130117, China)

  • Dexin Jin

    (School of Environment, Northeast Normal University, NO. 2555 Jingyue Street, Changchun 130117, China)

  • Jiao Qu

    (School of Environment, Northeast Normal University, NO. 2555 Jingyue Street, Changchun 130117, China)

  • Yanan Zhang

    (School of Environment, Northeast Normal University, NO. 2555 Jingyue Street, Changchun 130117, China)

Abstract

Dye effluent has attracted considerable attention from worldwide researchers due to its harm and toxicity in recent years; as a result, the treatment for dye has become one of the focuses in the environmental field. Adsorption has been widely applied in water treatment owing to its various advantages. However, the adsorption behaviors of the new materials, such as the 2D black phosphorus (BP), for pollution were urgently revealed and improved. In this work, BP, black phosphorene (BPR), and sulfonated BPR (BPRS) were prepared by the vapor phase deposition method, liquid-phase exfoliating method, and modification with sulfonation, respectively. The three BP-based materials were characterized and used as adsorbents for the removal of methylene blue (MB) in water. The results showed that the specific surface areas (SSAs) of BP, BPR, and BPRS were only 6.78, 6.92, and 7.72 m 2 ·g −1 , respectively. However, the maximum adsorption capacities of BP, BPR, and BPRS for MB could reach up to 84.03, 91.74, and 140.85 mg·g −1 , which were higher than other reported materials with large SSAs such as graphene (GP), nanosheet/magnetite, and reduced graphene oxide (rGO). In the process of BP adsorbing MB, wrinkles were generated, and the wrinkles would further induce adsorption. BPR had fewer layers (3–5), more wrinkles, and stronger adsorption capacity (91.74 mg·g −1 ). The interactions between the BP-based materials and MB might cause the BP-based materials to deform, i.e., to form wrinkles, thereby creating new adsorption sites between layers, and then further inducing adsorption. Although the wrinkles had a certain promotion effect, the adsorption capacity was limited, so the sulfonic acid functional group was introduced to modify BPR to increase its adsorption sites and promote the adsorption effect. These findings could provide a new viewpoint and insight on the adsorption behavior and potential application of the BP-based materials.

Suggested Citation

  • Juanhong Wang & Zhaocheng Zhang & Dongyang He & Hao Yang & Dexin Jin & Jiao Qu & Yanan Zhang, 2020. "Comparative Study on the Adsorption Capacities of the Three Black Phosphorus-Based Materials for Methylene Blue in Water," Sustainability, MDPI, vol. 12(20), pages 1-19, October.
    • Handle: RePEc:gam:jsusta:v:12:y:2020:i:20:p:8335-:d:425743
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    References listed on IDEAS

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    1. Jack P. C. Kleijnen, 2015. "Response Surface Methodology," International Series in Operations Research & Management Science, in: Michael C Fu (ed.), Handbook of Simulation Optimization, edition 127, chapter 0, pages 81-104, Springer.
    2. Fengnian Xia & Han Wang & Yichen Jia, 2014. "Rediscovering black phosphorus as an anisotropic layered material for optoelectronics and electronics," Nature Communications, Nature, vol. 5(1), pages 1-6, December.
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    Cited by:

    1. Ewa Okoniewska, 2021. "Removal of Selected Dyes on Activated Carbons," Sustainability, MDPI, vol. 13(8), pages 1-13, April.

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