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Study of a Li-Ion Cell Kinetics in Five Regions to Predict Li Plating Using a Pseudo Two-Dimensional Model

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  • Sanaz Momeni Boroujeni

    (Electrical Energy Storage Systems, Institute for Photovoltaics, University of Stuttgart, Pfaffenwaldring 47, 70569 Stuttgart, Germany)

  • Kai Peter Birke

    (Electrical Energy Storage Systems, Institute for Photovoltaics, University of Stuttgart, Pfaffenwaldring 47, 70569 Stuttgart, Germany)

Abstract

Detecting or predicting lithium plating in Li-ion cells and subsequently suppressing or preventing it have been the aim of many researches as it directly contributes to the aging, safety, and life-time of the cell. Although abundant influencing parameters on lithium deposition are already known, more information is still needed in order to predict this phenomenon and prevent it in time. It is observed that balancing in a Li-ion cell can play an important role in controlling lithium plating. In this work, five regions are defined with the intention of covering all the zones participating in the charge transfer from one electrode to the other during cell cycling. We employ a pseudo two-dimensional (P2D) cell model including two irreversible side reactions of solid electrolyte interface (SEI) formation and lithium plating (Li-P) as the anode aging mechanisms. With the help of simulated data and the Nernst–Einstein relation, ionic conductivities of the regions are calculated separately. Calculation results show that by aging the cell, more deviation between ionic conductivities of cathode and anode takes place which leads to the start of Li plating.

Suggested Citation

  • Sanaz Momeni Boroujeni & Kai Peter Birke, 2019. "Study of a Li-Ion Cell Kinetics in Five Regions to Predict Li Plating Using a Pseudo Two-Dimensional Model," Sustainability, MDPI, vol. 11(22), pages 1-14, November.
    • Handle: RePEc:gam:jsusta:v:11:y:2019:i:22:p:6392-:d:286680
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    References listed on IDEAS

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    1. Angeles Cabañero, Maria & Altmann, Johannes & Gold, Lukas & Boaretto, Nicola & Müller, Jana & Hein, Simon & Zausch, Jochen & Kallo, Josef & Latz, Arnulf, 2019. "Investigation of the temperature dependence of lithium plating onset conditions in commercial Li-ion batteries," Energy, Elsevier, vol. 171(C), pages 1217-1228.
    2. Eddahech, Akram & Briat, Olivier & Vinassa, Jean-Michel, 2013. "Thermal characterization of a high-power lithium-ion battery: Potentiometric and calorimetric measurement of entropy changes," Energy, Elsevier, vol. 61(C), pages 432-439.
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    4. Arminda Almeida & Nuno Sousa & João Coutinho-Rodrigues, 2019. "Quest for Sustainability: Life-Cycle Emissions Assessment of Electric Vehicles Considering Newer Li-Ion Batteries," Sustainability, MDPI, vol. 11(8), pages 1-19, April.
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    Cited by:

    1. Zhouting Sun & Mingyi Liu & Yong Zhu & Ruochen Xu & Zhiqiang Chen & Peng Zhang & Zeyu Lu & Pengcheng Wang & Chengrui Wang, 2022. "Issues Concerning Interfaces with Inorganic Solid Electrolytes in All-Solid-State Lithium Metal Batteries," Sustainability, MDPI, vol. 14(15), pages 1-23, July.

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