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Issues Concerning Interfaces with Inorganic Solid Electrolytes in All-Solid-State Lithium Metal Batteries

Author

Listed:
  • Zhouting Sun

    (Huaneng Clean Energy Research Institute, Beijing 102200, China)

  • Mingyi Liu

    (Huaneng Clean Energy Research Institute, Beijing 102200, China)

  • Yong Zhu

    (Huaneng Clean Energy Research Institute, Beijing 102200, China)

  • Ruochen Xu

    (Huaneng Clean Energy Research Institute, Beijing 102200, China)

  • Zhiqiang Chen

    (China Huaneng Group Hong Kong Limited, Hong Kong 100031, China)

  • Peng Zhang

    (China Huaneng Group Hong Kong Limited, Hong Kong 100031, China)

  • Zeyu Lu

    (China Huaneng Group Hong Kong Limited, Hong Kong 100031, China)

  • Pengcheng Wang

    (Huaneng Taishan New Energy Co. Ltd., Tai’an 271000, China)

  • Chengrui Wang

    (Huaneng Taishan New Energy Co. Ltd., Tai’an 271000, China)

Abstract

All-solid-state batteries have attracted wide attention for high-performance and safe batteries. The combination of solid electrolytes and lithium metal anodes makes high-energy batteries practical for next-generation high-performance devices. However, when a solid electrolyte replaces the liquid electrolyte, many different interface/interphase issues have arisen from the contact with electrodes. Poor wettability and unstable chemical/electrochemical reaction at the interfaces with lithium metal anodes will lead to poor lithium diffusion kinetics and combustion of fresh lithium and active materials in the electrolyte. Element cross-diffusion and charge layer formation at the interfaces with cathodes also impede the lithium ionic conductivity and increase the charge transfer resistance. The abovementioned interface issues hinder the electrochemical performance of all-solid-state lithium metal batteries. This review demonstrates the formation and mechanism of these interface issues between solid electrolytes and anodes/cathodes. Aiming to address the problems, we review and propose modification strategies to weaken interface resistance and improve the electrochemical performance of all-solid-state lithium metal batteries.

Suggested Citation

  • Zhouting Sun & Mingyi Liu & Yong Zhu & Ruochen Xu & Zhiqiang Chen & Peng Zhang & Zeyu Lu & Pengcheng Wang & Chengrui Wang, 2022. "Issues Concerning Interfaces with Inorganic Solid Electrolytes in All-Solid-State Lithium Metal Batteries," Sustainability, MDPI, vol. 14(15), pages 1-23, July.
    • Handle: RePEc:gam:jsusta:v:14:y:2022:i:15:p:9090-:d:870896
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    References listed on IDEAS

    as
    1. Sanaz Momeni Boroujeni & Kai Peter Birke, 2019. "Study of a Li-Ion Cell Kinetics in Five Regions to Predict Li Plating Using a Pseudo Two-Dimensional Model," Sustainability, MDPI, vol. 11(22), pages 1-14, November.
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    Cited by:

    1. Daems, K. & Yadav, P. & Dermenci, K.B. & Van Mierlo, J. & Berecibar, M., 2024. "Advances in inorganic, polymer and composite electrolytes: Mechanisms of Lithium-ion transport and pathways to enhanced performance," Renewable and Sustainable Energy Reviews, Elsevier, vol. 191(C).

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