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Recent Advances in Ball-Milling-Based Silicon Anodes for Lithium-Ion Batteries

Author

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  • Han Yang

    (School of Energy Sciences and Engineering, Nanjing Tech University, Nanjing 211816, China
    These authors contributed equally to this work.)

  • Shiyu Lin

    (School of Energy Sciences and Engineering, Nanjing Tech University, Nanjing 211816, China
    These authors contributed equally to this work.)

  • Alex Cheng

    (Shanghai Energy New Materials Technology Co., Ltd., Shanghai 201399, China)

  • Fangbo He

    (Zhuhai Energy New Materials Technology Co., Ltd., Zhuhai 519600, China)

  • Zhoulu Wang

    (School of Energy Sciences and Engineering, Nanjing Tech University, Nanjing 211816, China)

  • Yutong Wu

    (School of Energy Sciences and Engineering, Nanjing Tech University, Nanjing 211816, China)

  • Yi Zhang

    (School of Energy Sciences and Engineering, Nanjing Tech University, Nanjing 211816, China)

  • Xiang Liu

    (School of Energy Sciences and Engineering, Nanjing Tech University, Nanjing 211816, China)

Abstract

Having a high theoretical capacity density of 4200 mAh g −1 , silicon has been highlighted as one of the most promising anode materials for lithium-ion batteries. Countless silicon-based materials have been proposed and reported in research articles, mostly synthesized using bottom-up methods. While the infamous volume expansion issue can be settled with the bottom-up processes, the complicated protocols and high cost leave a non-neglectable gap between laboratory-scale and mass production. The top-down ball-milling method is still favored by industrial suppliers because of its simplicity and cost-effectiveness, even with compromised electrochemical performances. This paper reviews the latest development of ball-milling-based silicon anode materials. Although the ball-milling process seems straightforward, the procedures and parameters influencing the product have hardly been discussed in research papers compared to the bottom-up ones. This paper reviews recent advances in ball-milling-based silicon anode materials, provides a material comparison, and discusses how ball milling can provide lithium-ion batteries with greater possibilities at a larger scale.

Suggested Citation

  • Han Yang & Shiyu Lin & Alex Cheng & Fangbo He & Zhoulu Wang & Yutong Wu & Yi Zhang & Xiang Liu, 2023. "Recent Advances in Ball-Milling-Based Silicon Anodes for Lithium-Ion Batteries," Energies, MDPI, vol. 16(7), pages 1-21, March.
    • Handle: RePEc:gam:jeners:v:16:y:2023:i:7:p:3099-:d:1110240
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    References listed on IDEAS

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    1. Wangda Li & Evan M. Erickson & Arumugam Manthiram, 2020. "High-nickel layered oxide cathodes for lithium-based automotive batteries," Nature Energy, Nature, vol. 5(1), pages 26-34, January.
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