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Effect of electrode design and operating condition on performance of hydrogen alkaline membrane fuel cell

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  • Deng, Hao
  • Wang, Dawei
  • Wang, Renfang
  • Xie, Xu
  • Yin, Yan
  • Du, Qing
  • Jiao, Kui

Abstract

Hydrogen alkaline anion exchange membrane (AAEM) fuel cells are fabricated and tested, by measuring the output current densities at various cell voltages with a step change of 0.1V, under various ionomer contents in catalyst layer (volume fraction, 0.07, 0.21 and 0.50), inlet gas relative humidities (100%, 86% and 70%), anode back pressures (1.0, 1.01 and 1.02atm) and with/without insertion of micro porous layer (MPL). The corresponding theoretical analysis is also carried out, to clarify the factors that determine these experimental results. The experimental results show that high ionomer content, inlet gas humidity, slight anode pressurization and insertion of micro porous layer (MPL) are favorable. Since insufficient water supply (not oxygen) in cathode contributes to the major performance losses and low limiting current density, it is expected that properly increasing the water amount in cathode could effectively improve the membrane hydration, but not to causes considerable negative effect to cell performance.

Suggested Citation

  • Deng, Hao & Wang, Dawei & Wang, Renfang & Xie, Xu & Yin, Yan & Du, Qing & Jiao, Kui, 2016. "Effect of electrode design and operating condition on performance of hydrogen alkaline membrane fuel cell," Applied Energy, Elsevier, vol. 183(C), pages 1272-1278.
    • Handle: RePEc:eee:appene:v:183:y:2016:i:c:p:1272-1278
    DOI: 10.1016/j.apenergy.2016.09.091
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    1. Liu, Guicheng & Ding, Xianan & Zhou, Hongwei & Chen, Ming & Wang, Manxiang & Zhao, Zhenxuan & Yin, Zhuang & Wang, Xindong, 2015. "Structure optimization of cathode microporous layer for direct methanol fuel cells," Applied Energy, Elsevier, vol. 147(C), pages 396-401.
    2. Cho, Junhyun & Park, Jaeman & Oh, Hwanyeong & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2013. "Analysis of the transient response and durability characteristics of a proton exchange membrane fuel cell with different micro-porous layer penetration thicknesses," Applied Energy, Elsevier, vol. 111(C), pages 300-309.
    3. Deng, Hao & Wang, Dawei & Xie, Xu & Zhou, Yibo & Yin, Yan & Du, Qing & Jiao, Kui, 2016. "Modeling of hydrogen alkaline membrane fuel cell with interfacial effect and water management optimization," Renewable Energy, Elsevier, vol. 91(C), pages 166-177.
    4. Guo, Hang & Liu, Xuan & Zhao, Jian Fu & Ye, Fang & Ma, Chong Fang, 2014. "Experimental study of two-phase flow in a proton exchange membrane fuel cell in short-term microgravity condition," Applied Energy, Elsevier, vol. 136(C), pages 509-518.
    5. Chen, Ben & Ke, Wandi & Luo, Maji & Wang, Jun & Tu, Zhengkai & Pan, Mu & Zhang, Haining & Liu, Xiaowei & Liu, Wei, 2015. "Operation characteristics and carbon corrosion of PEMFC (Proton exchange membrane fuel cell) with dead-ended anode for high hydrogen utilization," Energy, Elsevier, vol. 91(C), pages 799-806.
    6. Park, Jaeman & Oh, Hwanyeong & Lee, Yoo Il & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2016. "Effect of the pore size variation in the substrate of the gas diffusion layer on water management and fuel cell performance," Applied Energy, Elsevier, vol. 171(C), pages 200-212.
    7. Yan, X.H. & Zhao, T.S. & An, L. & Zhao, G. & Zeng, L., 2015. "A crack-free and super-hydrophobic cathode micro-porous layer for direct methanol fuel cells," Applied Energy, Elsevier, vol. 138(C), pages 331-336.
    8. Oh, Hwanyeong & Park, Jaeman & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2015. "Effects of pore size gradient in the substrate of a gas diffusion layer on the performance of a proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 149(C), pages 186-193.
    9. Kong, Im Mo & Choi, Jong Won & Kim, Sung Il & Lee, Eun Sook & Kim, Min Soo, 2015. "Experimental study on the self-humidification effect in proton exchange membrane fuel cells containing double gas diffusion backing layer," Applied Energy, Elsevier, vol. 145(C), pages 345-353.
    10. Zeng, L. & Tang, Z.K. & Zhao, T.S., 2014. "A high-performance alkaline exchange membrane direct formate fuel cell," Applied Energy, Elsevier, vol. 115(C), pages 405-410.
    11. Xing, Lei & Das, Prodip K. & Song, Xueguan & Mamlouk, Mohamed & Scott, Keith, 2015. "Numerical analysis of the optimum membrane/ionomer water content of PEMFCs: The interaction of Nafion® ionomer content and cathode relative humidity," Applied Energy, Elsevier, vol. 138(C), pages 242-257.
    12. Zakaria, Z. & Kamarudin, S.K. & Timmiati, S.N., 2016. "Membranes for direct ethanol fuel cells: An overview," Applied Energy, Elsevier, vol. 163(C), pages 334-342.
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    Cited by:

    1. Wang, Bowen & Deng, Hao & Jiao, Kui, 2018. "Purge strategy optimization of proton exchange membrane fuel cell with anode recirculation," Applied Energy, Elsevier, vol. 225(C), pages 1-13.
    2. Cheng, Chaochao & Yang, Zirong & Liu, Zhi & Tongsh, Chasen & Zhang, Guobin & Xie, Biao & He, Shaoqing & Jiao, Kui, 2021. "Numerical investigation on the feasibility of metal foam as flow field in alkaline anion exchange membrane fuel cell," Applied Energy, Elsevier, vol. 302(C).
    3. Han, Chaoling & Chen, Zhenqian, 2021. "Study on the synergism of thermal transport and electrochemical of PEMFC based on N, P co-doped graphene substrate electrode," Energy, Elsevier, vol. 214(C).
    4. Noor H. Jawad & Ali Amer Yahya & Ali R. Al-Shathr & Hussein G. Salih & Khalid T. Rashid & Saad Al-Saadi & Adnan A. AbdulRazak & Issam K. Salih & Adel Zrelli & Qusay F. Alsalhy, 2022. "Fuel Cell Types, Properties of Membrane, and Operating Conditions: A Review," Sustainability, MDPI, vol. 14(21), pages 1-48, November.

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