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Carbon Dioxide Assisted Conversion of Hydrolysis Lignin Catalyzed by Nickel Compounds

Author

Listed:
  • Artem A. Medvedev

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia)

  • Daria A. Beldova

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia)

  • Konstantin B. Kalmykov

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia)

  • Alexey V. Kravtsov

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia)

  • Marina A. Tedeeva

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia)

  • Leonid M. Kustov

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia
    N.D. Zelinsky Institute of Organic Chemistry, Russian Academy of Sciences, Leninsky Prospect 47, 119991 Moscow, Russia
    Institute of Ecotechnologies and Engineering, National University of Science and Technology MISiS, Leninsky Prospect 4, 119991 Moscow, Russia)

  • Sergey F. Dunaev

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia)

  • Alexander L. Kustov

    (Chemistry Department, Moscow State University, 119992 Moscow, Russia
    N.D. Zelinsky Institute of Organic Chemistry, Russian Academy of Sciences, Leninsky Prospect 47, 119991 Moscow, Russia
    Institute of Ecotechnologies and Engineering, National University of Science and Technology MISiS, Leninsky Prospect 4, 119991 Moscow, Russia)

Abstract

In this work, hydrolysis lignin with nickel compounds deposited on the surface was prepared. The resulting material was introduced into the process of carbon dioxide assisted conversion and the catalytic activity of the deposited nickel compounds in this reaction was evaluated. Use of the obtained catalytic system increases CO 2 conversion by more than 30% in the temperature range 450–800 °C. After the conversion process, the material was subjected to a study using a variety of physico-chemical analysis methods (TEM, SEM-EDX, and X-ray phase analysis). Physico-chemical methods of analysis of a sample calcined at 300 °C to decompose nickel nitrate revealed NiO nanoparticles with an average particle size of 16.9 nm.

Suggested Citation

  • Artem A. Medvedev & Daria A. Beldova & Konstantin B. Kalmykov & Alexey V. Kravtsov & Marina A. Tedeeva & Leonid M. Kustov & Sergey F. Dunaev & Alexander L. Kustov, 2022. "Carbon Dioxide Assisted Conversion of Hydrolysis Lignin Catalyzed by Nickel Compounds," Energies, MDPI, vol. 15(18), pages 1-12, September.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:18:p:6774-:d:916818
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    References listed on IDEAS

    as
    1. Chio, Chonlong & Sain, Mohini & Qin, Wensheng, 2019. "Lignin utilization: A review of lignin depolymerization from various aspects," Renewable and Sustainable Energy Reviews, Elsevier, vol. 107(C), pages 232-249.
    2. Zhang, Fan & Xu, Deping & Wang, Yonggang & Argyle, Morris D. & Fan, Maohong, 2015. "CO2 gasification of Powder River Basin coal catalyzed by a cost-effective and environmentally friendly iron catalyst," Applied Energy, Elsevier, vol. 145(C), pages 295-305.
    3. Won-Ju Lee & Dae-Young Kim & Jae-Hyuk Choi & Ji-Woong Lee & Jun-Soo Kim & Kwangho Son & Min-Jae Ha & Jun Kang, 2019. "Utilization of Petroleum Coke Soot as Energy Storage Material," Energies, MDPI, vol. 12(16), pages 1-9, August.
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