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Evolution of Internal Stress in Heterogeneous Electrode Composite during the Drying Process

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  • Zuoquan Zhu

    (Shanghai Institute of Applied Mathematics and Mechanics, School of Mechanics and Engineering Science, Shanghai University, Shanghai 200444, China
    Shanghai Key Laboratory of Mechanics in Energy Engineering, Shanghai 200072, China)

  • Yaolong He

    (Shanghai Institute of Applied Mathematics and Mechanics, School of Mechanics and Engineering Science, Shanghai University, Shanghai 200444, China
    Shanghai Key Laboratory of Mechanics in Energy Engineering, Shanghai 200072, China
    Shaoxing Institute of Technology, Shanghai University, Shanghai 200072, China)

  • Hongjiu Hu

    (Shanghai Institute of Applied Mathematics and Mechanics, School of Mechanics and Engineering Science, Shanghai University, Shanghai 200444, China
    Shanghai Key Laboratory of Mechanics in Energy Engineering, Shanghai 200072, China)

  • Fangzhou Zhang

    (Shaoxing Institute of Technology, Shanghai University, Shanghai 200072, China
    Institute of Materials, Shanghai University, Shanghai 200072, China)

Abstract

The mechanical behavior of electrode composite during the drying preparation has played a crucial role in the electrochemical performance of lithium-ion batteries (LIBs). Our work aimed at developing an integrated analysis method to study the component distribution, mechanical properties, and internal stress of composite coating in the process of electrode drying. The main influence factors of drying stress were thoroughly investigated. It was found that this present model could capture not only the heterogeneity effect of inactive ingredients but also the porosity-dependent viscoelasticity of electrode composite. Meanwhile, the calculated effective modulus and stress evolution upon drying time were in acceptable accord with the experimental data. Furthermore, the rapid solidification markedly increased the drying stress in electrodes and significantly impaired the tensile strength of electrode composite due to the highly gradient distributed constituents. However, the stress level at high drying temperature could be significantly reduced by an aqueous sodium alginate binder instead of poly(vinylidene fluoride). The obtained results will be a great help in efficiently manufacturing LIB electrodes with adequate mechanical integrity.

Suggested Citation

  • Zuoquan Zhu & Yaolong He & Hongjiu Hu & Fangzhou Zhang, 2021. "Evolution of Internal Stress in Heterogeneous Electrode Composite during the Drying Process," Energies, MDPI, vol. 14(6), pages 1-15, March.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:6:p:1683-:d:519516
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    References listed on IDEAS

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    1. M. Armand & J.-M. Tarascon, 2008. "Building better batteries," Nature, Nature, vol. 451(7179), pages 652-657, February.
    2. Arno Kwade & Wolfgang Haselrieder & Ruben Leithoff & Armin Modlinger & Franz Dietrich & Klaus Droeder, 2018. "Current status and challenges for automotive battery production technologies," Nature Energy, Nature, vol. 3(4), pages 290-300, April.
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    Cited by:

    1. João C. Barbosa & Renato Gonçalves & Carlos M. Costa & Senentxu Lanceros-Mendez, 2021. "Recent Advances on Materials for Lithium-Ion Batteries," Energies, MDPI, vol. 14(11), pages 1-36, May.

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