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Enhanced performance and lifetime of lithium-ion batteries by laser structuring of graphite anodes

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  • Kriegler, Johannes
  • Hille, Lucas
  • Stock, Sandro
  • Kraft, Ludwig
  • Hagemeister, Jan
  • Habedank, Jan Bernd
  • Jossen, Andreas
  • Zaeh, Michael F.

Abstract

Improving the performance characteristics of lithium-ion batteries is a central research objective for the widespread introduction of electric vehicles. Laser-induced structures in graphite anodes have been reported to improve various performance characteristics of lithium-ion batteries. Nevertheless, electrode structuring has been studied mostly with single-layer coin cells on a laboratory scale to date. In addition to electrochemical tests on multi-layer NMC111/graphite pouch cells with a nominal capacity of ≈ 2.9 Ah, this paper presents the transfer of the technology from the laboratory to an industry-oriented battery production scale. A significant improvement of the discharge rate capability of lithium-ion batteries with laser-structured anodes was observed at temperatures of -10 °C, 0 °C, and 25 °C at discharge rates of up to 8C. Moreover, an enhanced fast-charging capability at charge rates as high as 6C was determined. In an aging study with 500 charge and discharge cycles, a significantly higher capacity retention of cells containing structured anodes was demonstrated. The effects of aging were investigated by incremental capacity analyses. Additionally, the results are supported by post-mortem analyses of the anode material using scanning electron microscopy and energy-dispersive X-ray spectroscopy. The investigations revealed a distinctly reduced surface layer formation on structured anodes in comparison to their non-structured counterparts, which is attributed to a decrease in lithium-plating during cycling.

Suggested Citation

  • Kriegler, Johannes & Hille, Lucas & Stock, Sandro & Kraft, Ludwig & Hagemeister, Jan & Habedank, Jan Bernd & Jossen, Andreas & Zaeh, Michael F., 2021. "Enhanced performance and lifetime of lithium-ion batteries by laser structuring of graphite anodes," Applied Energy, Elsevier, vol. 303(C).
    • Handle: RePEc:eee:appene:v:303:y:2021:i:c:s0306261921010539
    DOI: 10.1016/j.apenergy.2021.117693
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    References listed on IDEAS

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    1. Zubi, Ghassan & Dufo-López, Rodolfo & Carvalho, Monica & Pasaoglu, Guzay, 2018. "The lithium-ion battery: State of the art and future perspectives," Renewable and Sustainable Energy Reviews, Elsevier, vol. 89(C), pages 292-308.
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    1. He, Rong & He, Yongling & Xie, Wenlong & Guo, Bin & Yang, Shichun, 2023. "Comparative analysis for commercial li-ion batteries degradation using the distribution of relaxation time method based on electrochemical impedance spectroscopy," Energy, Elsevier, vol. 263(PD).
    2. Shen, Yudong & Wang, Xueyuan & Jiang, Zhao & Luo, Bingyin & Chen, Daidai & Wei, Xuezhe & Dai, Haifeng, 2024. "Online detection of lithium plating onset during constant and multistage constant current fast charging for lithium-ion batteries," Applied Energy, Elsevier, vol. 370(C).

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