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Effect of the Presence of HCl on Simultaneous CO 2 Capture and Contaminants Removal from Simulated Biomass Gasification Producer Gas by CaO-Fe 2 O 3 Sorbent in Calcium Looping Cycles

Author

Listed:
  • Forogh Dashtestani

    (Department of Chemical and Process Engineering, University of Canterbury, Christchurch 8041, New Zealand)

  • Mohammad Nusheh

    (Hot Lime Labs, Lower Hutt 5040, New Zealand)

  • Vilailuck Siriwongrungson

    (College of Advanced Manufacturing Innovation, King Mongkut’s Institute of Technology Ladkrabang, Bangkok 10520, Thailand)

  • Janjira Hongrapipat

    (Gussing Renewable Energy (Thailand) Co., Ltd., Bangkok 10500, Thailand)

  • Vlatko Materic

    (Hot Lime Labs, Lower Hutt 5040, New Zealand)

  • Alex C. K. Yip

    (Department of Chemical and Process Engineering, University of Canterbury, Christchurch 8041, New Zealand)

  • Shusheng Pang

    (Department of Chemical and Process Engineering, University of Canterbury, Christchurch 8041, New Zealand)

Abstract

This study investigated the effect of HCl in biomass gasification producer gas on the CO 2 capture efficiency and contaminants removal efficiency by CaO-Fe 2 O 3 based sorbent material in the calcium looping process. Experiments were conducted in a fixed bed reactor to capture CO 2 from the producer gas with the combined contaminants of HCl at 200 ppmv, H 2 S at 230 ppmv, and NH 3 at 2300 ppmv. The results show that with presence of HCl in the feeding gas, sorbent reactivity for CO 2 capture and contaminants removal was enhanced. The maximum CO 2 capture was achieved at carbonation temperatures of 680 °C, with efficiencies of 93%, 92%, and 87%, respectively, for three carbonation-calcination cycles. At this carbonation temperature, the average contaminant removal efficiencies were 92.7% for HCl, 99% for NH 3 , and 94.7% for H 2 S. The outlet contaminant concentrations during the calcination process were also examined which is useful for CO 2 reuse. The pore structure change of the used sorbent material suggests that the HCl in the feeding gas contributes to high CO 2 capture efficiency and contaminants removal simultaneously.

Suggested Citation

  • Forogh Dashtestani & Mohammad Nusheh & Vilailuck Siriwongrungson & Janjira Hongrapipat & Vlatko Materic & Alex C. K. Yip & Shusheng Pang, 2021. "Effect of the Presence of HCl on Simultaneous CO 2 Capture and Contaminants Removal from Simulated Biomass Gasification Producer Gas by CaO-Fe 2 O 3 Sorbent in Calcium Looping Cycles," Energies, MDPI, vol. 14(23), pages 1-12, December.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:23:p:8167-:d:695832
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    1. Wang, Wenjing & Li, Yingjie & Xie, Xin & Sun, Rongyue, 2014. "Effect of the presence of HCl on cyclic CO2 capture of calcium-based sorbent in calcium looping process," Applied Energy, Elsevier, vol. 125(C), pages 246-253.
    2. Guillermo Martinez Castilla & Diana Carolina Guío-Pérez & Stavros Papadokonstantakis & David Pallarès & Filip Johnsson, 2021. "Techno-Economic Assessment of Calcium Looping for Thermochemical Energy Storage with CO 2 Capture," Energies, MDPI, vol. 14(11), pages 1-17, May.
    3. Perejón, Antonio & Romeo, Luis M. & Lara, Yolanda & Lisbona, Pilar & Martínez, Ana & Valverde, Jose Manuel, 2016. "The Calcium-Looping technology for CO2 capture: On the important roles of energy integration and sorbent behavior," Applied Energy, Elsevier, vol. 162(C), pages 787-807.
    4. Erans, María & Manovic, Vasilije & Anthony, Edward J., 2016. "Calcium looping sorbents for CO2 capture," Applied Energy, Elsevier, vol. 180(C), pages 722-742.
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