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Performance and Durability of the Zr-Doped CaO Sorbent under Cyclic Carbonation–Decarbonation at Different Operating Parameters

Author

Listed:
  • Vyacheslav V. Rodaev

    (Institute for Nanotechnology and Nanomaterials, Derzhavin Tambov State University, Internatsionalnaya Str. 33, 392000 Tambov, Russia)

  • Svetlana S. Razlivalova

    (Institute for Nanotechnology and Nanomaterials, Derzhavin Tambov State University, Internatsionalnaya Str. 33, 392000 Tambov, Russia)

Abstract

The effect of cyclic carbonation–decarbonation operating parameters on Zr-doped CaO sorbent CO 2 uptake capacity evolution is examined. It is revealed that the capacity steady state value increases with the decrease in the carbonation temperature, CO 2 concentration in the gas flow upon carbonation and with the increase in the heating rate from the carbonation to the decarbonation stages. The rise in decarbonation temperature leads to a dramatic decrease in the sorbent performance. It is found that if carbonation occurs at 630 °C in the gas flow containing 15 vol.% CO 2 and decarbonation is carried out at 742 °C, the sorbent shows the highest values of the initial and steady state CO 2 uptake capacity, namely, 10.7 mmol/g and 9.4 mmol/g, respectively.

Suggested Citation

  • Vyacheslav V. Rodaev & Svetlana S. Razlivalova, 2021. "Performance and Durability of the Zr-Doped CaO Sorbent under Cyclic Carbonation–Decarbonation at Different Operating Parameters," Energies, MDPI, vol. 14(16), pages 1-9, August.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:16:p:4822-:d:610327
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    References listed on IDEAS

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    1. Antzara, Andy & Heracleous, Eleni & Lemonidou, Angeliki A., 2015. "Improving the stability of synthetic CaO-based CO2 sorbents by structural promoters," Applied Energy, Elsevier, vol. 156(C), pages 331-343.
    2. Antonio Coppola & Fabrizio Scala, 2020. "A Preliminary Techno-Economic Analysis on the Calcium Looping Process with Simultaneous Capture of CO 2 and SO 2 from a Coal-Based Combustion Power Plant," Energies, MDPI, vol. 13(9), pages 1-9, May.
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