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A Comparative Study of Using Polarization Curve Models in Proton Exchange Membrane Fuel Cell Degradation Analysis

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  • Chen Zhang

    (Department of Precision Machinery and Precision Instrumentation, University of Science and Technology of China, Hefei 230026, China)

  • Wen Li

    (Department of Thermal Science and Energy Engineering, University of Science and Technology of China, Hefei 230026, China)

  • Mingruo Hu

    (School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai 200240, China)

  • Xiaofang Cheng

    (Department of Thermal Science and Energy Engineering, University of Science and Technology of China, Hefei 230026, China)

  • Kai He

    (Department of Precision Machinery and Precision Instrumentation, University of Science and Technology of China, Hefei 230026, China)

  • Lei Mao

    (Department of Precision Machinery and Precision Instrumentation, University of Science and Technology of China, Hefei 230026, China)

Abstract

In this paper, a systematic study is carried out to compare the performance of various V-I models at both normal and faulty conditions, in terms of simulating proton exchange membrane fuel cell (PEMFC) behavior and analyzing the corresponding degradation process. In the analysis, the simulation accuracy of V-I models, including overall behavior simulation and the simulation of different PEMFC losses, is investigated. Results show that compared to the other V-I models, the V-I model using exponential function for mass transport loss and considering open circuit voltage (OCV) at zero current can provide the best simulation performance, with an overall root mean square error (RMSE) of about 0.00279. Furthermore, the performance of these V-I models in analyzing PEMFC degradation process is also studied. By investigating the evolution of PEMFC losses during the degradation, the effectiveness of these models in interpreting PEMFC degradation mechanisms can be clarified. The results show that, besides the simulation accuracy, different interpretations may be provided from different models; this further confirms the necessity of comparative study. Moreover, the effectiveness of different V-I models in identifying PEMFC abnormal performance at two faulty scenarios is investigated. The results demonstrate that, among different V-I models, the model using an exponential function for mass transport loss and considering OCV at zero current can provide more accurate simulation and reasonable interpretation regarding PEMFC internal behavior.

Suggested Citation

  • Chen Zhang & Wen Li & Mingruo Hu & Xiaofang Cheng & Kai He & Lei Mao, 2020. "A Comparative Study of Using Polarization Curve Models in Proton Exchange Membrane Fuel Cell Degradation Analysis," Energies, MDPI, vol. 13(15), pages 1-16, July.
    • Handle: RePEc:gam:jeners:v:13:y:2020:i:15:p:3759-:d:387989
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    References listed on IDEAS

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    1. Priya, K. & Sathishkumar, K. & Rajasekar, N., 2018. "A comprehensive review on parameter estimation techniques for Proton Exchange Membrane fuel cell modelling," Renewable and Sustainable Energy Reviews, Elsevier, vol. 93(C), pages 121-144.
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    2. Khadijeh Hooshyari & Bahman Amini Horri & Hamid Abdoli & Mohsen Fallah Vostakola & Parvaneh Kakavand & Parisa Salarizadeh, 2021. "A Review of Recent Developments and Advanced Applications of High-Temperature Polymer Electrolyte Membranes for PEM Fuel Cells," Energies, MDPI, vol. 14(17), pages 1-38, September.
    3. Ewa Janicka & Michal Mielniczek & Lukasz Gawel & Kazimierz Darowicki, 2021. "Optimization of the Relative Humidity of Reactant Gases in Hydrogen Fuel Cells Using Dynamic Impedance Measurements," Energies, MDPI, vol. 14(11), pages 1-11, May.
    4. Huu Linh Nguyen & Jeasu Han & Xuan Linh Nguyen & Sangseok Yu & Young-Mo Goo & Duc Dung Le, 2021. "Review of the Durability of Polymer Electrolyte Membrane Fuel Cell in Long-Term Operation: Main Influencing Parameters and Testing Protocols," Energies, MDPI, vol. 14(13), pages 1-34, July.

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