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Characterization and kinetics of iron oxide reduction by corn straw biochar prepared by pyrolysis using superheated steam atmosphere and hydrothermal processes

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  • Han, Chengjin
  • Wei, Guangsheng
  • Zhu, Rong
  • Cheng, Yu
  • Wang, Runzhe
  • Wu, Wenhe
  • Wang, Yefeng

Abstract

Current research on using biochar as foaming agents in electric arc furnace (EAF) steelmaking is limited to pyrolysis biochar treated with nitrogen. Therefore, this study used pyrolysis corn stalk biochar treated with nitrogen (PN) as a reference, the physical and chemical properties, the ability to reduce iron oxide, and the reaction mechanism of pyrolysis corn stalk biochar treated with superheated steam (PSS) and hydrothermal corn stalk biochar (HC) were investigated. HC contains a large number of hydrogen-containing functional groups, which can release large amounts of H2 during the reduction of iron oxide, while PSS has a higher fixed carbon content and produces higher amounts of CO and CO2 gas. Dividing the thermogravimetric results into three reduction stages, the results show that the large amount of volatile fraction contained in HC contributes to Stage 1 and that the gasification reaction ability of PSS is stronger than that of PN. The results of the kinetic analysis showed that the best reaction mechanism for the three reduction stages of the three biochars was the Jander diffusion equation. This work provides theoretical guidance for the use of PSS and HC as foaming agents in EAF steelmaking.

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  • Han, Chengjin & Wei, Guangsheng & Zhu, Rong & Cheng, Yu & Wang, Runzhe & Wu, Wenhe & Wang, Yefeng, 2023. "Characterization and kinetics of iron oxide reduction by corn straw biochar prepared by pyrolysis using superheated steam atmosphere and hydrothermal processes," Renewable Energy, Elsevier, vol. 219(P2).
    • Handle: RePEc:eee:renene:v:219:y:2023:i:p2:s0960148123014866
    DOI: 10.1016/j.renene.2023.119571
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    References listed on IDEAS

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    1. Dhyani, Vaibhav & Bhaskar, Thallada, 2018. "A comprehensive review on the pyrolysis of lignocellulosic biomass," Renewable Energy, Elsevier, vol. 129(PB), pages 695-716.
    2. Ren, Lei & Zhou, Sheng & Peng, Tianduo & Ou, Xunmin, 2021. "A review of CO2 emissions reduction technologies and low-carbon development in the iron and steel industry focusing on China," Renewable and Sustainable Energy Reviews, Elsevier, vol. 143(C).
    3. Raza, Mohsin & Abu-Jdayil, Basim & Al-Marzouqi, Ali H. & Inayat, Abrar, 2022. "Kinetic and thermodynamic analyses of date palm surface fibers pyrolysis using Coats-Redfern method," Renewable Energy, Elsevier, vol. 183(C), pages 67-77.
    4. Kambo, Harpreet Singh & Dutta, Animesh, 2015. "A comparative review of biochar and hydrochar in terms of production, physico-chemical properties and applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 45(C), pages 359-378.
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    1. Hu, Bo & Xu, Lianfei & Li, Yang & Sun, Fei & Wang, Zhuozhi & Yang, Mengchi & Zhang, Yangyang & Kong, Wenwen & Shen, Boxiong & Wang, Xin & Yang, Jiancheng, 2024. "Biochar and Fe2+ mediation in hydrogen production by water electrolysis: Effects of physicochemical properties of biochars," Energy, Elsevier, vol. 297(C).

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