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Effect of structural characteristics and surface functional groups of biochar on thermal properties of different organic phase change materials: Dominant encapsulation mechanisms

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  • Lv, Laiquan
  • Wang, Jiankang
  • Ji, Mengting
  • Zhang, Yize
  • Huang, Shengyao
  • Cen, Kefa
  • Zhou, Hao

Abstract

In this article, waste phoenix leaf biochar was introduced into three most used organic phase change materials (PCMs) to prepare shape-stable composite PCMs by the vacuum impregnation method. The encapsulation capacity and encapsulation efficiency of steam activated biochar for paraffin, stearic acid, and polyethylene glycol were 59.28% and 49.14%, 63.03% and 57.62%, 71.38% and 46.84%, respectively, which was related to the mechanisms of biochar encapsulated organic PCMs. The dominant mechanisms of biochar encapsulated organic PCMs are summarized as pore-filling, hydrogen-bonding, hydrophobic interaction between biochar and PCMs, and other potential mechanisms. Influence degree η was introduced to illustrate the effect of biochar on organic PCMs, 16.56%, 8.72%, and 35.75% for steam activated biochar on paraffin, stearic acid, and polyethylene glycol. In addition, compared with original PCMs, the thermal conductivity of biochar-based composite PCMs first decreased and then increased with the increase of biochar pyrolysis temperature. Moreover, biochar-based composite PCMs had better thermal stability, concerned with the dominant mechanisms of biochar encapsulated organic PCMs. Therefore, biochar-based composite PCMs proposed in this study expand the application of biochar and organic PCMs in thermal energy storage, building energy conservation, solar energy utilization, and battery thermal management system.

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  • Lv, Laiquan & Wang, Jiankang & Ji, Mengting & Zhang, Yize & Huang, Shengyao & Cen, Kefa & Zhou, Hao, 2022. "Effect of structural characteristics and surface functional groups of biochar on thermal properties of different organic phase change materials: Dominant encapsulation mechanisms," Renewable Energy, Elsevier, vol. 195(C), pages 1238-1252.
    • Handle: RePEc:eee:renene:v:195:y:2022:i:c:p:1238-1252
    DOI: 10.1016/j.renene.2022.06.117
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    2. Yin, Qianqian & Zhu, Ge & Wang, Ruikun & Zhao, Zhenghui, 2024. "Enhancing the thermal storage performance of biochar/paraffin composite phase change materials: Effect of oleophobic modification of biochar," Energy, Elsevier, vol. 293(C).
    3. Lv, Laiquan & Huang, Shengyao & Zou, Yang & Wang, Xinyi & Zhou, Hao, 2024. "Thermal performance investigation of a medium-temperature pilot-scale latent heat thermal energy storage system: The constant and step temperatures charging and discharging," Renewable Energy, Elsevier, vol. 225(C).
    4. Amelia Carolina Sparavigna, 2023. "Multifunctional Porosity in Biochar," International Journal of Sciences, Office ijSciences, vol. 12(07), pages 41-54, July.
    5. Huang, Xinyu & Li, Fangfei & Liu, Zhengguang & Gao, Xinyu & Yang, Xiaohu & Yan, Jinyue, 2023. "Design and optimization of a novel phase change photovoltaic thermal utilization structure for building envelope," Renewable Energy, Elsevier, vol. 218(C).

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