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Three-dimensional hierarchical porous carbon surface-decorated graphitic carbon foam/stearic acid composite as high-performance shape-stabilized phase change material with desirable photothermal conversion efficiency

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  • Zhou, Yunhong
  • Zeng, Jiwei
  • Guo, Yiyou
  • Chen, Haobin
  • Bi, Tiantian
  • Lin, Qilang

Abstract

To simultaneously improve the photothermal conversion and encapsulation capacity of phase change material (PCM), a three-dimensional hierarchical porous carbon surface-decorated graphitic carbon foam (SGF) was developed. Employing this SGF as an encapsulated skeleton for stearic acid (SA), a unique shape-stabilized SA/SGF composite PCM was successfully prepared after vacuum impregnation. The porous carbon surface exhibits a uniform and fluffy three-dimensional continuous network structure well adhered onto the pore walls of the SGF; it can act as a desirable interfacial layer between SA and the SGF, which gives the composite effective encapsulation performance and good interfacial compatibility. The as-prepared composite has a loading capacity of 78.16% for melted SA without any leakage, and possesses a thermal conductivity of 3.25 W/mK with 1377% higher than that of SA and a compressive strength of 4.41 MPa (increasing 283.5% than the SGF). Further, the melting and crystallization enthalpy of the composite reaches 167.6 J/g and 167.5 J/g, respectively, with a thermal storage efficiency of up to 95.13%; meanwhile, it displays excellent thermal cycle stability revealed by keeping an enthalpy of 92.80% after 200 thermal cycles. More importantly, it presents a high photothermal conversion of 90.14% at 200 mW/cm2 with the ability to serve as a stable heat source during solar-thermal-electric conversion. Consequently, the composite has great potential in solar storage and waste heat recycle.

Suggested Citation

  • Zhou, Yunhong & Zeng, Jiwei & Guo, Yiyou & Chen, Haobin & Bi, Tiantian & Lin, Qilang, 2023. "Three-dimensional hierarchical porous carbon surface-decorated graphitic carbon foam/stearic acid composite as high-performance shape-stabilized phase change material with desirable photothermal conve," Applied Energy, Elsevier, vol. 352(C).
    • Handle: RePEc:eee:appene:v:352:y:2023:i:c:s0306261923013594
    DOI: 10.1016/j.apenergy.2023.121995
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