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Transformation of residual fatty raw materials into third generation green diesel over a nickel catalyst supported on mineral palygorskite

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  • Lycourghiotis, Sotiris
  • Kordouli, Eleana
  • Kordulis, Christos
  • Bourikas, Kyriakos

Abstract

The transformation of residual fatty raw materials (RFRMs) (waste cooking oils (WCO), fatty acid distillate (FAD), oil extracted from spent coffee grounds (SCGO) and oil from chicken fat (CHO)) into third generation green diesel was studied over a very active nickel catalyst supported on mineral palygorskite. The transformation of biodiesel into green diesel was also studied. The physicochemical characteristics of the RFRMs were correlated with their composition and the conditions and procedure of their preparation. The composition of the reaction liquid mixture in total green diesel follows the order: 98% (CHO), 83% (WCO), 68% (FAD) and 10% (SCGO). Biodiesel is transformed much faster into green diesel than RFRMs. The catalyst use does not affect its main physicochemical characteristics. The activity trend was rationalized in terms of the relative surface concentrations of the supported nickel phases and on the basis of some molecules present in the RFRMs which may bring about catalyst deactivation.

Suggested Citation

  • Lycourghiotis, Sotiris & Kordouli, Eleana & Kordulis, Christos & Bourikas, Kyriakos, 2021. "Transformation of residual fatty raw materials into third generation green diesel over a nickel catalyst supported on mineral palygorskite," Renewable Energy, Elsevier, vol. 180(C), pages 773-786.
    • Handle: RePEc:eee:renene:v:180:y:2021:i:c:p:773-786
    DOI: 10.1016/j.renene.2021.08.059
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    2. Tsiotsias, Anastasios I. & Hafeez, Sanaa & Charisiou, Nikolaos D. & Al-Salem, Sultan M. & Manos, George & Constantinou, Achilleas & AlKhoori, Sara & Sebastian, Victor & Hinder, Steven J. & Baker, Mark, 2023. "Selective catalytic deoxygenation of palm oil to produce green diesel over Ni catalysts supported on ZrO2 and CeO2–ZrO2: Experimental and process simulation modelling studies," Renewable Energy, Elsevier, vol. 206(C), pages 582-596.
    3. Stefania Lucantonio & Andrea Di Giuliano & Leucio Rossi & Katia Gallucci, 2023. "Green Diesel Production via Deoxygenation Process: A Review," Energies, MDPI, vol. 16(2), pages 1-44, January.
    4. Wang, Fei & Xu, Hui & Yu, Songyin & Zhu, Hao & Du, Yuchan & Zhang, Zeng & You, Chaoqun & Jiang, Xiaoxiang & Jiang, Jianchun, 2022. "Fe-promoted Ni catalyst with extremely high loading and oxygen vacancy for lipid deoxygenation into green diesel," Renewable Energy, Elsevier, vol. 197(C), pages 40-49.

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