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Electrochemical conversion of CO2 into tunable syngas on a B, P, N tri-doped carbon

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  • Han, Juan
  • Deng, Ximing
  • Chen, Keyu
  • Imhanria, Sarah
  • Sun, Yan
  • Wang, Wei

Abstract

The fabrication of syngas by CO2 reduction reaction (CO2RR) can avoid the disadvantages of its traditional industrial productions that exacerbate energy crisis and environmental problems. Herein, a series of B, P, N tri-doped carbon (BPNC) catalysts are developed for CO2RR. The results show that, the products of CO2 electroreduction on as-prepared BPNC are CO and H2 with no other products. And on the optimal BPNC (1000 °C, nC48H40BP: nmelamine = 1:200), the faradaic efficiency of CO can reach 81.8 %, with the ratio of H2/CO from 0.2 to 6.8 easily regulated by controlling the applied potential during CO2RR process. This study would provide a good option for production of tunable syngas feedstock by CO2RR process using carbon-based catalysts for numerous downstream processes.

Suggested Citation

  • Han, Juan & Deng, Ximing & Chen, Keyu & Imhanria, Sarah & Sun, Yan & Wang, Wei, 2021. "Electrochemical conversion of CO2 into tunable syngas on a B, P, N tri-doped carbon," Renewable Energy, Elsevier, vol. 177(C), pages 636-642.
    • Handle: RePEc:eee:renene:v:177:y:2021:i:c:p:636-642
    DOI: 10.1016/j.renene.2021.06.001
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    1. Jingjie Wu & Sichao Ma & Jing Sun & Jake I. Gold & ChandraSekhar Tiwary & Byoungsu Kim & Lingyang Zhu & Nitin Chopra & Ihab N. Odeh & Robert Vajtai & Aaron Z. Yu & Raymond Luo & Jun Lou & Guqiao Ding , 2016. "A metal-free electrocatalyst for carbon dioxide reduction to multi-carbon hydrocarbons and oxygenates," Nature Communications, Nature, vol. 7(1), pages 1-6, December.
    2. Jin-Woong Lee & Woon Bae Park & Jin Hee Lee & Satendra Pal Singh & Kee-Sun Sohn, 2020. "A deep-learning technique for phase identification in multiphase inorganic compounds using synthetic XRD powder patterns," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    3. Hanif, Saadia & Iqbal, Naseem & Shi, Xuan & Noor, Tayyaba & Ali, Ghulam & Kannan, A.M., 2020. "NiCo–N-doped carbon nanotubes based cathode catalyst for alkaline membrane fuel cell," Renewable Energy, Elsevier, vol. 154(C), pages 508-516.
    4. Wang, Chao & Wang, Hanwei & Dang, Baokang & Wang, Zhe & Shen, Xiaoping & Li, Caicai & Sun, Qingfeng, 2020. "Ultrahigh yield of nitrogen doped porous carbon from biomass waste for supercapacitor," Renewable Energy, Elsevier, vol. 156(C), pages 370-376.
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