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Ultrahigh yield of nitrogen doped porous carbon from biomass waste for supercapacitor

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  • Wang, Chao
  • Wang, Hanwei
  • Dang, Baokang
  • Wang, Zhe
  • Shen, Xiaoping
  • Li, Caicai
  • Sun, Qingfeng

Abstract

Conversion of Biomass into porous carbon with high yield is a huge challenge due to the consumption of plentiful carbon during pore-forming. Here, we employ the biomass materials as the activation agent to circumvent the excessive etching effect of the conventional chemical reagent. Both green activation agent and raw material are converted into porous carbon, which results in ultrahigh yield (even more than 100%). Furthermore, the biomass activation agent with abundant metal elements not only contributes to pore-forming but also achieves heteroatom doping. The obtained N-doped hierarchical porous carbon presented good capacitive capability (150.1 F g−1 at 0.2 A g−1) and high rate performance (∼61% of capacitance retention from 0.2 to 50 A g−1). The green activation process achieves both the increase of yield and excellent capacitive properties for the first time. The green strategy proposed in this work for producing porous carbon with high yield provides a new consideration on comprehensive utilization of biomass resources.

Suggested Citation

  • Wang, Chao & Wang, Hanwei & Dang, Baokang & Wang, Zhe & Shen, Xiaoping & Li, Caicai & Sun, Qingfeng, 2020. "Ultrahigh yield of nitrogen doped porous carbon from biomass waste for supercapacitor," Renewable Energy, Elsevier, vol. 156(C), pages 370-376.
    • Handle: RePEc:eee:renene:v:156:y:2020:i:c:p:370-376
    DOI: 10.1016/j.renene.2020.04.092
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    1. Abioye, Adekunle Moshood & Ani, Farid Nasir, 2015. "Recent development in the production of activated carbon electrodes from agricultural waste biomass for supercapacitors: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 52(C), pages 1282-1293.
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    2. Wang, Xiaoxiang & Cao, Li & Lewis, Rosmala & Hreid, Tubuxin & Zhang, Zhanying & Wang, Hongxia, 2020. "Biorefining of sugarcane bagasse to fermentable sugars and surface oxygen group-rich hierarchical porous carbon for supercapacitors," Renewable Energy, Elsevier, vol. 162(C), pages 2306-2317.
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    4. Han, Juan & Deng, Ximing & Chen, Keyu & Imhanria, Sarah & Sun, Yan & Wang, Wei, 2021. "Electrochemical conversion of CO2 into tunable syngas on a B, P, N tri-doped carbon," Renewable Energy, Elsevier, vol. 177(C), pages 636-642.
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    9. Ozpinar, Pelin & Dogan, Ceren & Demiral, Hakan & Morali, Ugur & Erol, Salim & Samdan, Canan & Yildiz, Derya & Demiral, Ilknur, 2022. "Activated carbons prepared from hazelnut shell waste by phosphoric acid activation for supercapacitor electrode applications and comprehensive electrochemical analysis," Renewable Energy, Elsevier, vol. 189(C), pages 535-548.
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