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Ultrahigh yield of nitrogen doped porous carbon from biomass waste for supercapacitor

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  • Wang, Chao
  • Wang, Hanwei
  • Dang, Baokang
  • Wang, Zhe
  • Shen, Xiaoping
  • Li, Caicai
  • Sun, Qingfeng

Abstract

Conversion of Biomass into porous carbon with high yield is a huge challenge due to the consumption of plentiful carbon during pore-forming. Here, we employ the biomass materials as the activation agent to circumvent the excessive etching effect of the conventional chemical reagent. Both green activation agent and raw material are converted into porous carbon, which results in ultrahigh yield (even more than 100%). Furthermore, the biomass activation agent with abundant metal elements not only contributes to pore-forming but also achieves heteroatom doping. The obtained N-doped hierarchical porous carbon presented good capacitive capability (150.1 F g−1 at 0.2 A g−1) and high rate performance (∼61% of capacitance retention from 0.2 to 50 A g−1). The green activation process achieves both the increase of yield and excellent capacitive properties for the first time. The green strategy proposed in this work for producing porous carbon with high yield provides a new consideration on comprehensive utilization of biomass resources.

Suggested Citation

  • Wang, Chao & Wang, Hanwei & Dang, Baokang & Wang, Zhe & Shen, Xiaoping & Li, Caicai & Sun, Qingfeng, 2020. "Ultrahigh yield of nitrogen doped porous carbon from biomass waste for supercapacitor," Renewable Energy, Elsevier, vol. 156(C), pages 370-376.
    • Handle: RePEc:eee:renene:v:156:y:2020:i:c:p:370-376
    DOI: 10.1016/j.renene.2020.04.092
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    References listed on IDEAS

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    1. Abioye, Adekunle Moshood & Ani, Farid Nasir, 2015. "Recent development in the production of activated carbon electrodes from agricultural waste biomass for supercapacitors: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 52(C), pages 1282-1293.
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    2. Yuan, Xiangzhou & Wang, Junyao & Deng, Shuai & Suvarna, Manu & Wang, Xiaonan & Zhang, Wei & Hamilton, Sara Triana & Alahmed, Ammar & Jamal, Aqil & Park, Ah-Hyung Alissa & Bi, Xiaotao & Ok, Yong Sik, 2022. "Recent advancements in sustainable upcycling of solid waste into porous carbons for carbon dioxide capture," Renewable and Sustainable Energy Reviews, Elsevier, vol. 162(C).
    3. Han, Juan & Deng, Ximing & Chen, Keyu & Imhanria, Sarah & Sun, Yan & Wang, Wei, 2021. "Electrochemical conversion of CO2 into tunable syngas on a B, P, N tri-doped carbon," Renewable Energy, Elsevier, vol. 177(C), pages 636-642.
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    5. Li, Dong & Guo, Yanchuan & Li, Yi & Liu, Zhengang & Chen, Zeliang, 2022. "Waste-biomass tar functionalized carbon spheres with N/P Co-doping and hierarchical pores as sustainable low-cost energy storage materials," Renewable Energy, Elsevier, vol. 188(C), pages 61-69.
    6. Qin, Liyuan & Wu, Yang & Jiang, Enchen, 2022. "In situ template preparation of porous carbon materials that are derived from swine manure and have ordered hierarchical nanopore structures for energy storage," Energy, Elsevier, vol. 242(C).
    7. Wang, Xiaoxiang & Cao, Li & Lewis, Rosmala & Hreid, Tubuxin & Zhang, Zhanying & Wang, Hongxia, 2020. "Biorefining of sugarcane bagasse to fermentable sugars and surface oxygen group-rich hierarchical porous carbon for supercapacitors," Renewable Energy, Elsevier, vol. 162(C), pages 2306-2317.
    8. Xia, Guoyan & Liu, Zhanglin & He, Jinsong & Huang, Mei & Zhao, Li & Zou, Jianmei & Lei, Yongjia & Yang, Qiulin & Liu, Yan & Tian, Dong & Shen, Fei, 2024. "Modulating three-dimensional porous carbon from paper mulberry juice by a hydrothermal process for a supercapacitor with excellent performance," Renewable Energy, Elsevier, vol. 227(C).
    9. Zhu, Lingyan & Liu, Xudong & Wu, Yuan & Wang, Qifan & Wang, Haotian & Li, Dongbing, 2022. "Fast-pyrolysis lignin-biochar as an excellent precursor for high-performance capacitors," Renewable Energy, Elsevier, vol. 198(C), pages 1318-1327.
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