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Fast pyrolysis of biomass in a spouted bed reactor: Hydrodynamics, heat transfer and chemical reaction

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  • Park, Hoon Chae
  • Choi, Hang Seok

Abstract

The present study focused on modeling the gas-solid multi-phase flow and pyrolysis reaction of biomass in a spouted bed reactor. For the first time, the kinetics of biomass pyrolysis in a spouted bed were measured by the micro-spouted bed thermogravimetric analyzer (MSB-TGA) and applied to the fast pyrolysis reaction during computational particle fluid dynamics (CPFD) analysis. The CPFD results of biomass pyrolysis show that, compared to conventional TGA, the kinetic data obtained by MSB-TGA provide reliable results for the pyrolysis reaction of biomass. The effects of reaction temperature and gas velocity on hydrodynamics, heat transfer, and the consequent pyrolysis reaction were also investigated. A significant change in pyrolysis product yield was observed as a result of enhanced mixing and heat transfer between bed materials and biomass particles by increasing the gas velocity. The tar yield increased to 64.8 wt% when the gas velocity was increased to 6 m/s, and then it decreased as the gas velocity exceeded 6 m/s. With increasing reaction temperature, the tar yield first increased and then decreased, with a maximum value of approximately 58.7 wt% at 450 °C. From 450 to 550 °C, the tar yield decreased from 58.7 wt% to 50.9 wt%, respectively.

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  • Park, Hoon Chae & Choi, Hang Seok, 2019. "Fast pyrolysis of biomass in a spouted bed reactor: Hydrodynamics, heat transfer and chemical reaction," Renewable Energy, Elsevier, vol. 143(C), pages 1268-1284.
    • Handle: RePEc:eee:renene:v:143:y:2019:i:c:p:1268-1284
    DOI: 10.1016/j.renene.2019.05.072
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    References listed on IDEAS

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    1. Butler, Eoin & Devlin, Ger & Meier, Dietrich & McDonnell, Kevin, 2011. "A review of recent laboratory research and commercial developments in fast pyrolysis and upgrading," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(8), pages 4171-4186.
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    1. Sang Kyu Choi & Yeon Seok Choi & Yeon Woo Jeong & So Young Han & Quynh Van Nguyen, 2020. "Simulation of the Fast Pyrolysis of Coffee Ground in a Tilted-Slide Reactor," Energies, MDPI, vol. 13(24), pages 1-19, December.
    2. Yang, Shiliang & Fan, Feihu & Hu, Jianhang & Wang, Hua, 2020. "Particle-scale evaluation of the biomass steam-gasification process in a conical spouted bed gasifier," Renewable Energy, Elsevier, vol. 162(C), pages 844-860.
    3. Anirudh Kulkarni & Garima Mishra & Sridhar Palla & Potnuri Ramesh & Dadi Venkata Surya & Tanmay Basak, 2023. "Advances in Computational Fluid Dynamics Modeling for Biomass Pyrolysis: A Review," Energies, MDPI, vol. 16(23), pages 1-32, November.
    4. Sun, Haoran & Yang, Shiliang & Bao, Guirong & Hu, Jianhang & Wang, Hua, 2023. "Numerical evaluation of multi-scale properties in biomass fast pyrolysis in fountain confined conical spouted bed," Energy, Elsevier, vol. 283(C).
    5. Yang, Shiliang & Dong, Ruihan & Du, Yanxiang & Wang, Shuai & Wang, Hua, 2021. "Numerical study of the biomass pyrolysis process in a spouted bed reactor through computational fluid dynamics," Energy, Elsevier, vol. 214(C).

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