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Co-gasification of coal and biomass blends using dolomite and olivine as catalysts

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  • Ma, Xinyue
  • Zhao, Xue
  • Gu, Jiyou
  • Shi, Junyou

Abstract

Natural catalysts (dolomite and olivine) not only reduce the tar content, they also have a high potential to enhance hydrogen production during gasification process. In this study, a bubbling fluidized bed (BFB) was used to evaluate the effect of the operating parameters on co-gasification of pine sawdust and brown coal namely gasification temperature (Tg) in the range of 700–1000 °C, fuel particle size (dp) in the range of 2.0–3.5 mm, steam/fuel ratio (S/F) in the range of 0.5–0.8, equivalence ratio (ER) in the range of 0.1–0.4, biomass ratio (BR) in the range of 0.0–100%, and catalyst loading in the range of 3.0–12.0 wt%. With increase in catalyst loading from 3.0 to 12.0 (wt %), the hydrogen yield was increased from 52.9 to 55.5 (g/kg-fuel) for dolomite and from 47.5 to 52.1 (g/kg-fuel) for olivine, while the tar yield sharply decreased from 5.4 to 0.4 (g/Nm3) and from 7.0 to 0.8 (g/Nm3), respectively. Fuel particle size showed a negligible influence on the upgrading of hydrogen production and tar yield.

Suggested Citation

  • Ma, Xinyue & Zhao, Xue & Gu, Jiyou & Shi, Junyou, 2019. "Co-gasification of coal and biomass blends using dolomite and olivine as catalysts," Renewable Energy, Elsevier, vol. 132(C), pages 509-514.
    • Handle: RePEc:eee:renene:v:132:y:2019:i:c:p:509-514
    DOI: 10.1016/j.renene.2018.07.077
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    1. Devi, Lopamudra & Ptasinski, Krzysztof J. & Janssen, Frans J.J.G. & van Paasen, Sander V.B. & Bergman, Patrick C.A. & Kiel, Jacob H.A., 2005. "Catalytic decomposition of biomass tars: use of dolomite and untreated olivine," Renewable Energy, Elsevier, vol. 30(4), pages 565-587.
    2. W. A. Wan Ab Karim Ghani & Reza Alipour Moghadam & M. A. Mohd Salleh & A. B. Alias, 2009. "Air Gasification of Agricultural Waste in a Fluidized Bed Gasifier: Hydrogen Production Performance," Energies, MDPI, vol. 2(2), pages 1-11, May.
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    5. Zhang, Heng & Li, Junguo & Yang, Xin & Song, Shuangshuang & Wang, Zhiqing & Huang, Jiejie & Zhang, Yongqi & Fang, Yitian, 2020. "Influence of coal ash on CO2 gasification reactivity of corn stalk char," Renewable Energy, Elsevier, vol. 147(P1), pages 2056-2063.
    6. Inayat, Muddasser & Sulaiman, Shaharin A. & Kurnia, Jundika Candra & Shahbaz, Muhammad, 2019. "Effect of various blended fuels on syngas quality and performance in catalytic co-gasification: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 105(C), pages 252-267.
    7. Zhang, Guozhao & Liu, Hao & Wang, Jia & Wu, Baojia, 2018. "Catalytic gasification characteristics of rice husk with calcined dolomite," Energy, Elsevier, vol. 165(PB), pages 1173-1177.
    8. Chen, Guan-Bang & Wu, Fang-Hsien & Lin, Sheng-Pin & Hsu, Yun-Ting & Lin, Ta-Hui, 2022. "A study of sewage sludge Co-gasification with waste shiitake substrate," Energy, Elsevier, vol. 259(C).
    9. Kamble, Alka D. & Mendhe, Vinod A. & Chavan, Prakash D. & Saxena, Vinod K., 2022. "Insights of mineral catalytic effects of high ash coal on carbon conversion in fluidized bed Co-gasification through FTIR, XRD, XRF and FE-SEM," Renewable Energy, Elsevier, vol. 183(C), pages 729-751.

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    Keywords

    Olivine; Dolomite; Biomass; Coal; Hydrogen; Tar;
    All these keywords.

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