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Type of contribution: Research article catalytic activity of sewage sludge char supported Re-Ni bimetallic catalyst toward cracking/reforming of biomass tar

Author

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  • Daorattanachai, Pornlada
  • Laosiripojana, Weerawan
  • Laobuthee, Apirat
  • Laosiripojana, Navadol

Abstract

In the present work, catalytic activities of sewage sludge char supported Re-Ni bimetallic catalyst toward cracking/reforming of naphthalene and biomass tar were studied. Several proportions of Re and Ni (i.e. 1:9, 3:7, 5:5, 7:3 and 9:1) were investigated and their activities were compared to char, Ni/char and Re/char catalysts. Among all catalysts, the highest naphthalene cracking conversion and H2 yield were achieved from Re-Ni/char with Re:Ni ratio of 3:7. From the post-reaction characterizations, the additional of Re into Ni not only improves the dispersion of Ni on char surface by preventing agglomeration of particles but also improve the catalyst resistance toward carbon deposition. The additional of steam and O2 along with naphthalene as steam and autothermal reforming were also carried out. The presences of suitable steam and O2 can further promote H2 production and significantly reduce the degree of carbon formation. Under optimum conditions at 800 °C with H2O/C and O2/C molar ratios of 1.5 and 0.3, the catalyst exhibited high biomass tar conversion with only 5% deactivation in H2 yield after 18 h operation. Therefore, this study indicates the successful development of catalyst and process for biomass tar conversion via cracking and reforming processes.

Suggested Citation

  • Daorattanachai, Pornlada & Laosiripojana, Weerawan & Laobuthee, Apirat & Laosiripojana, Navadol, 2018. "Type of contribution: Research article catalytic activity of sewage sludge char supported Re-Ni bimetallic catalyst toward cracking/reforming of biomass tar," Renewable Energy, Elsevier, vol. 121(C), pages 644-651.
  • Handle: RePEc:eee:renene:v:121:y:2018:i:c:p:644-651
    DOI: 10.1016/j.renene.2018.01.096
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    References listed on IDEAS

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    1. Shen, Yafei, 2015. "Chars as carbonaceous adsorbents/catalysts for tar elimination during biomass pyrolysis or gasification," Renewable and Sustainable Energy Reviews, Elsevier, vol. 43(C), pages 281-295.
    2. Guan, Guoqing & Kaewpanha, Malinee & Hao, Xiaogang & Abudula, Abuliti, 2016. "Catalytic steam reforming of biomass tar: Prospects and challenges," Renewable and Sustainable Energy Reviews, Elsevier, vol. 58(C), pages 450-461.
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    1. Gu, Jing & Wang, Shuxiao & Lu, Tao & Wu, Yufeng & Yuan, Haoran & Chen, Yong, 2020. "Synthesis and evaluation of pyrolysis waste peat char supported catalyst for steam reforming of toluene," Renewable Energy, Elsevier, vol. 160(C), pages 964-973.
    2. Čespiva, Jakub & Wnukowski, Mateusz & Niedzwiecki, Lukasz & Skřínský, Jan & Vereš, Ján & Ochodek, Tadeáš & Pawlak-Kruczek, Halina & Borovec, Karel, 2020. "Characterization of tars from a novel, pilot scale, biomass gasifier working under low equivalence ratio regime," Renewable Energy, Elsevier, vol. 159(C), pages 775-785.
    3. Wang, Shuxiao & Zhang, Yuyuan & Shan, Rui & Gu, Jing & Yuan, Haoran & Chen, Yong, 2022. "Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production," Energy, Elsevier, vol. 246(C).
    4. Ramesh, Arumugam & Tamizhdurai, Perumal & Shanthi, Kannan, 2019. "Catalytic hydrodeoxygenation of jojoba oil to the green-fuel application on Ni-MoS/Mesoporous zirconia-silica catalysts," Renewable Energy, Elsevier, vol. 138(C), pages 161-173.
    5. Wang, Shuxiao & Shan, Rui & Lu, Tao & Zhang, Yuyuan & Yuan, Haoran & Chen, Yong, 2020. "Pyrolysis char derived from waste peat for catalytic reforming of tar model compound," Applied Energy, Elsevier, vol. 263(C).
    6. Li, Longzhi & Yang, Zhijuan & Qin, Xiaomin & Chen, Jian & Yan, Keshuo & Zou, Guifu & Peng, Zhuoyan & Wang, Fumao & Song, Zhanlong & Ma, Chunyuan, 2019. "Toluene microwave-assisted reforming with CO2 or a mixed agent of CO2-H2O on Fe-doped activated biochar," Energy, Elsevier, vol. 177(C), pages 358-366.
    7. Thongkumkoon, Skonrach & Kiatkittipong, Worapon & Hartley, Unalome Wetwatana & Laosiripojana, Navadol & Daorattanachai, Pornlada, 2019. "Catalytic activity of trimetallic sulfided Re-Ni-Mo/γ-Al2O3 toward deoxygenation of palm feedstocks," Renewable Energy, Elsevier, vol. 140(C), pages 111-123.
    8. Shen, Yafei & Zhou, Yuewei & Fu, Yuhong & Zhang, Niyu, 2020. "Activated carbons synthesized from unaltered and pelletized biomass wastes for bio-tar adsorption in different phases," Renewable Energy, Elsevier, vol. 146(C), pages 1700-1709.
    9. Li, Longzhi & Meng, Bo & Qin, Xiaomin & Yang, Zhijuan & Chen, Jian & Yan, Keshuo & Wang, Fumao, 2020. "Toluene microwave cracking and reforming over bio-char with in-situ activation and ex-situ impregnation of metal," Renewable Energy, Elsevier, vol. 149(C), pages 1205-1213.

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