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A combined methanol autothermal steam reforming and PEM fuel cell pilot plant unit: Experimental and simulation studies

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  • Ouzounidou, Martha
  • Ipsakis, Dimitris
  • Voutetakis, Spyros
  • Papadopoulou, Simira
  • Seferlis, Panos

Abstract

An integrated system for hydrogen production via autothermal steam reforming of methanol and consequent power generation in a polymer electrolyte membrane (PEM) fuel cell has been developed and operated at C.P.E.R.I. The pilot plant comprises an autothermal reforming reactor to produce hydrogen, a preferential oxidation reactor (PROX) to reduce CO concentration below 50ppm and a PEM fuel cell for power generation.

Suggested Citation

  • Ouzounidou, Martha & Ipsakis, Dimitris & Voutetakis, Spyros & Papadopoulou, Simira & Seferlis, Panos, 2009. "A combined methanol autothermal steam reforming and PEM fuel cell pilot plant unit: Experimental and simulation studies," Energy, Elsevier, vol. 34(10), pages 1733-1743.
    • Handle: RePEc:eee:energy:v:34:y:2009:i:10:p:1733-1743
    DOI: 10.1016/j.energy.2009.06.031
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    References listed on IDEAS

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    Cited by:

    1. Salemme, Lucia & Menna, Laura & Simeone, Marino, 2013. "Calculation of the energy efficiency of fuel processor – PEM (proton exchange membrane) fuel cell systems from fuel elementar composition and heating value," Energy, Elsevier, vol. 57(C), pages 368-374.
    2. Zhang, Xiuqin & Guo, Juncheng & Chen, Jincan, 2010. "The parametric optimum analysis of a proton exchange membrane (PEM) fuel cell and its load matching," Energy, Elsevier, vol. 35(12), pages 5294-5299.
    3. Khadijeh Hooshyari & Bahman Amini Horri & Hamid Abdoli & Mohsen Fallah Vostakola & Parvaneh Kakavand & Parisa Salarizadeh, 2021. "A Review of Recent Developments and Advanced Applications of High-Temperature Polymer Electrolyte Membranes for PEM Fuel Cells," Energies, MDPI, vol. 14(17), pages 1-38, September.
    4. Lesmana, Donny & Wu, Ho-Shing, 2014. "Modified oxalic acid co-precipitation method for preparing Cu/ZnO/Al2O3/Cr2O3/CeO2 catalysts for the OR (oxidative reforming) of M (methanol) to produce H2 (hydrogen) gas," Energy, Elsevier, vol. 69(C), pages 769-777.
    5. Zhang, Tie-qing & Malik, Fawad Rahim & Jung, Seunghun & Kim, Young-Bae, 2022. "Hydrogen production and temperature control for DME autothermal reforming process," Energy, Elsevier, vol. 239(PA).
    6. Iulianelli, A. & Ribeirinha, P. & Mendes, A. & Basile, A., 2014. "Methanol steam reforming for hydrogen generation via conventional and membrane reactors: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 29(C), pages 355-368.
    7. Ipsakis, Dimitris & Ouzounidou, Martha & Papadopoulou, Simira & Seferlis, Panos & Voutetakis, Spyros, 2017. "Dynamic modeling and control analysis of a methanol autothermal reforming and PEM fuel cell power system," Applied Energy, Elsevier, vol. 208(C), pages 703-718.
    8. Wang, Feng & Cao, Yiding & Wang, Guoqiang, 2015. "Thermoelectric generation coupling methanol steam reforming characteristic in microreactor," Energy, Elsevier, vol. 80(C), pages 642-653.
    9. Garcia, Gabriel & Arriola, Emmanuel & Chen, Wei-Hsin & De Luna, Mark Daniel, 2021. "A comprehensive review of hydrogen production from methanol thermochemical conversion for sustainability," Energy, Elsevier, vol. 217(C).
    10. Yuan, Zhenyu & Zhang, Yufeng & Fu, Wenting & Li, Zipeng & Liu, Xiaowei, 2013. "Investigation of a small-volume direct methanol fuel cell stack for portable applications," Energy, Elsevier, vol. 51(C), pages 462-467.
    11. Tie-Qing Zhang & Seunghun Jung & Young-Bae Kim, 2022. "Hydrogen Production System through Dimethyl Ether Autothermal Reforming, Based on Model Predictive Control," Energies, MDPI, vol. 15(23), pages 1-16, November.
    12. Authayanun, Suthida & Saebea, Dang & Patcharavorachot, Yaneeporn & Arpornwichanop, Amornchai, 2014. "Effect of different fuel options on performance of high-temperature PEMFC (proton exchange membrane fuel cell) systems," Energy, Elsevier, vol. 68(C), pages 989-997.
    13. Inbamrung, Piyanut & Sornchamni, Thana & Prapainainar, Chaiwat & Tungkamani, Sabaithip & Narataruksa, Phavanee & Jovanovic, Goran N., 2018. "Modeling of a square channel monolith reactor for methane steam reforming," Energy, Elsevier, vol. 152(C), pages 383-400.
    14. Samuel Simon Araya & Søren Juhl Andreasen & Søren Knudsen Kær, 2012. "Experimental Characterization of the Poisoning Effects of Methanol-Based Reformate Impurities on a PBI-Based High Temperature PEM Fuel Cell," Energies, MDPI, vol. 5(11), pages 1-17, October.
    15. Lee, Jun Sung & Han, Gi Bo & Kang, Misook, 2012. "Low temperature steam reforming of ethanol for carbon monoxide-free hydrogen production over mesoporous Sn-incorporated SBA-15 catalysts," Energy, Elsevier, vol. 44(1), pages 248-256.
    16. Yao, Ling & Wang, Feng & Wang, Long & Wang, Guoqiang, 2019. "Transport enhancement study on small-scale methanol steam reforming reactor with waste heat recovery for hydrogen production," Energy, Elsevier, vol. 175(C), pages 986-997.
    17. Lee, Chun-Boo & Cho, Sung-Ho & Lee, Dong-Wook & Hwang, Kyung-Ran & Park, Jong-Soo & Kim, Sung-Hyun, 2014. "Combination of preferential CO oxidation and methanation in hybrid MCR (micro-channel reactor) for CO clean-up," Energy, Elsevier, vol. 78(C), pages 421-425.
    18. Authayanun, Suthida & Saebea, Dang & Patcharavorachot, Yaneeporn & Arpornwichanop, Amornchai, 2015. "Evaluation of an integrated methane autothermal reforming and high-temperature proton exchange membrane fuel cell system," Energy, Elsevier, vol. 80(C), pages 331-339.

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