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A novel water perm-selective membrane dual-type reactor concept for Fischer–Tropsch synthesis of GTL (gas to liquid) technology

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  • Rahimpour, M.R.
  • Mirvakili, A.
  • Paymooni, K.

Abstract

The present study proposes a novel configuration of Fischer–Tropsch synthesis (FTS) reactors in which a fixed-bed water perm-selective membrane reactor is followed by a fluidized-bed hydrogen perm-selective membrane reactor. This novel concept which has been named fixed-bed membrane reactor followed by fluidized-bed membrane reactor (FMFMDR) produces gasoline from synthesis gas. The walls of the tubes of a fixed-bed reactor (water-cooled reactor) of FMFMDR configuration are coated by a high water perm-selective membrane layer. In this new configuration, two membrane reactors instead of one membrane reactor are developed for FTS reactions. In other words, two different membrane layers are used. In order to investigate the performance of FMFMDR, a one-dimensional heterogeneous model is taken into consideration. The simulation results of three schemes named fluidized-bed membrane dual-type reactor (FMDR), FMFMDR and conventional fixed-bed reactor (CR) are presented. They have been compared in terms of temperature, gasoline and CO2 yields, H2 and CO conversions and the water permeation rate through the membrane layer. Results show that the gasoline yield in FMFMDR is higher than the one in FMDR. The FMFMDR configuration not only decreases the undesired product such as CO2 but also produces more gasoline.

Suggested Citation

  • Rahimpour, M.R. & Mirvakili, A. & Paymooni, K., 2011. "A novel water perm-selective membrane dual-type reactor concept for Fischer–Tropsch synthesis of GTL (gas to liquid) technology," Energy, Elsevier, vol. 36(2), pages 1223-1235.
    • Handle: RePEc:eee:energy:v:36:y:2011:i:2:p:1223-1235
    DOI: 10.1016/j.energy.2010.11.023
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    References listed on IDEAS

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    2. Bakhtyari, Ali & Bardool, Roghayeh & Rahimpour, Mohammad Reza & Iulianelli, Adolfo, 2021. "Dehydration of bio-alcohols in an enhanced membrane-assisted reactor: A rigorous sensitivity analysis and multi-objective optimization," Renewable Energy, Elsevier, vol. 177(C), pages 519-543.
    3. Wang, Guoqiang & Wang, Feng & Li, Longjian & Zhang, Guofu, 2013. "Experiment of catalyst activity distribution effect on methanol steam reforming performance in the packed bed plate-type reactor," Energy, Elsevier, vol. 51(C), pages 267-272.
    4. Zohdi-Fasaei, Hossein & Atashi, Hossein & Farshchi Tabrizi, Farshad & Mirzaei, Ali Akbar, 2017. "Modeling and optimization of Fischer-Tropsch synthesis over Co-Mn-Ce/SiO2 catalyst using hybrid RSM/LHHW approaches," Energy, Elsevier, vol. 128(C), pages 496-508.

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