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Catalytic co-pyrolysis of poplar tree and polystyrene with HZSM-5 and Fe/HZSM-5 for production of light aromatic hydrocarbons

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  • Guo, Shuaihua
  • Wang, Zhiwei
  • Chen, Gaofeng
  • Chen, Yan
  • Wu, Mengge
  • Zhang, Mengju
  • Li, Zaifeng
  • Yang, Shuhua
  • Lei, Tingzhou

Abstract

The catalytic co-pyrolysis of biomass and plastic waste is a highly effective approach for the production of light aromatic hydrocarbons. In this study, catalytic co-pyrolysis experiments were conducted on poplar tree (PT) and polystyrene (PS) using pyrolyzer coupled with gas chromatography/mass spectrometry (Py-GC/MS). The experiments were carried out at a temperature of 550 °C and a mixing ratio of 1:1. X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), and scanning electron microscopy (SEM) techniques were employed for the characterization of HZSM-5 and Fe/HZSM-5 catalysts. The findings indicated that the metallic Fe in the HZSM-5 catalyst led to an enhanced production of monocyclic aromatic hydrocarbons (MAH) during the catalytic co-pyrolysis of PT and PS. The proportion of MAH in the products obtained from HZSM-5 and Fe/HZSM-5 catalyst was determined to be 85.84 % and 90.87 %, respectively. In the catalytic co-pyrolysis of biomass and plastic waste, several crucial reactions took place, including deoxidation, olefins aromatization, and Diels-Alder reaction between furans and olefins. In the presence of Fe metal, the HZSM-5 catalyst exhibited enhanced selectivity towards valuable MAH while effectively suppressing the formation of polycyclic aromatic hydrocarbons, resulting in an increase in MAH production to 90.87 %.

Suggested Citation

  • Guo, Shuaihua & Wang, Zhiwei & Chen, Gaofeng & Chen, Yan & Wu, Mengge & Zhang, Mengju & Li, Zaifeng & Yang, Shuhua & Lei, Tingzhou, 2024. "Catalytic co-pyrolysis of poplar tree and polystyrene with HZSM-5 and Fe/HZSM-5 for production of light aromatic hydrocarbons," Energy, Elsevier, vol. 298(C).
    • Handle: RePEc:eee:energy:v:298:y:2024:i:c:s0360544224012064
    DOI: 10.1016/j.energy.2024.131433
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    References listed on IDEAS

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