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Functional groups anchoring-induced Ni/MoOx-Ov interface on rice husk char for hydrodeoxygenation of bio-guaiacol to BTX at ambient-pressure

Author

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  • Fan, Xudong
  • Wu, Yujian
  • Sun, Yan
  • Tu, Ren
  • Ren, Zhipeng
  • Liang, Kaili
  • Jiang, Enchen
  • Ren, Yongzhi
  • Xu, Xiwei

Abstract

Bio-char is a promising carrier for the catalysts applied in hydrodeoxygenation (HDO) of bio-oil. The impact of bio-char surface microenvironment on the active phase needs to be further explored. In this work, O-containing functional groups were employed in adjusting the surface microenvironment of biomass-derived char with Ni–Mo loading. And the effect of geometric structure and electronic modification of Ni/MoOx-Ov interface on the atmospheric HDO activity of guaiacol over Ni-MoOx/bio-char catalyst was studied. Multiple characterizations revealed that the O-containing functional groups on bio-char carriers not only promoted the dispersion of active metals, but also decreased the particle size, thus resulting in the boosting of Ni/MoOx-Ov interface. Moreover, the intrinsic active sites were sumi-quantitatively analyzed via H2-TPD, and a positive correlation was established between BTX yield and quantity of Ni/MoOx-Ov interface. Furthermore, the effects of hydrothermal parameters for preparing bio-char, HDO conditions (temperature, WHSV and stability) and the metal loadings on the catalytic performance of Ni-MoOx/bio-char catalysts were studied in detail. This work provides a theoretical support to develop cost-effective catalysts with the utilization of biomass waste material.

Suggested Citation

  • Fan, Xudong & Wu, Yujian & Sun, Yan & Tu, Ren & Ren, Zhipeng & Liang, Kaili & Jiang, Enchen & Ren, Yongzhi & Xu, Xiwei, 2022. "Functional groups anchoring-induced Ni/MoOx-Ov interface on rice husk char for hydrodeoxygenation of bio-guaiacol to BTX at ambient-pressure," Renewable Energy, Elsevier, vol. 200(C), pages 579-591.
    • Handle: RePEc:eee:renene:v:200:y:2022:i:c:p:579-591
    DOI: 10.1016/j.renene.2022.09.080
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    References listed on IDEAS

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    1. Lee, Jechan & Kim, Ki-Hyun & Kwon, Eilhann E., 2017. "Biochar as a Catalyst," Renewable and Sustainable Energy Reviews, Elsevier, vol. 77(C), pages 70-79.
    2. Fan, Xu-dong & Wu, Yu-jian & Tu, Ren & Sun, Yan & Jiang, En-chen & Xu, Xi-wei, 2020. "Hydrodeoxygenation of guaiacol via rice husk char supported Ni based catalysts: The influence of char supports," Renewable Energy, Elsevier, vol. 157(C), pages 1035-1045.
    3. Bhoi, P.R. & Ouedraogo, A.S. & Soloiu, V. & Quirino, R., 2020. "Recent advances on catalysts for improving hydrocarbon compounds in bio-oil of biomass catalytic pyrolysis," Renewable and Sustainable Energy Reviews, Elsevier, vol. 121(C).
    4. Wu, Yujian & Xu, Xiwei & Sun, Yan & Jiang, Enchen & Fan, Xudong & Tu, Ren & Wang, Jiamin, 2020. "Gas-phase hydrodeoxygenation of guaiacol over Ni-based HUSY zeolite catalysts under atmospheric H2 pressure," Renewable Energy, Elsevier, vol. 152(C), pages 1380-1390.
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    1. Gollakota, Anjani R.K. & Shu, Chi-Min & Sarangi, Prakash Kumar & Shadangi, Krushna Prasad & Rakshit, Sudip & Kennedy, John F. & Gupta, Vijai Kumar & Sharma, Minaxi, 2023. "Catalytic hydrodeoxygenation of bio-oil and model compounds - Choice of catalysts, and mechanisms," Renewable and Sustainable Energy Reviews, Elsevier, vol. 187(C).

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