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Optimization of synthesis gas production in the biomass chemical looping gasification process operating under auto-thermal conditions

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  • Samprón, Iván
  • de Diego, Luis F.
  • García-Labiano, Francisco
  • Izquierdo, María T.

Abstract

Biomass Chemical Looping Gasification (BCLG) is a promising route to obtain N2 free high purity syngas. In this work, heat and mass balances were solved to determine the auto-thermal operation conditions that maximize the syngas yield in a BCLG system. A Fe-based oxygen carrier and pine wood as fuel were considered for the simulation. Two methods to control the transference of oxygen between the air reactor (AR) and fuel reactor (FR) were analysed. Syngas yield was higher controlling the oxygen fed to the AR by the air flow (OCM-1) than controlling the oxygen supplied to the FR by the oxygen carrier circulation flow (OCM-2).

Suggested Citation

  • Samprón, Iván & de Diego, Luis F. & García-Labiano, Francisco & Izquierdo, María T., 2021. "Optimization of synthesis gas production in the biomass chemical looping gasification process operating under auto-thermal conditions," Energy, Elsevier, vol. 226(C).
    • Handle: RePEc:eee:energy:v:226:y:2021:i:c:s0360544221005661
    DOI: 10.1016/j.energy.2021.120317
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    References listed on IDEAS

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    1. Huang, Zhen & He, Fang & Zhu, Huangqing & Chen, Dezhen & Zhao, Kun & Wei, Guoqiang & Feng, Yipeng & Zheng, Anqing & Zhao, Zengli & Li, Haibin, 2015. "Thermodynamic analysis and thermogravimetric investigation on chemical looping gasification of biomass char under different atmospheres with Fe2O3 oxygen carrier," Applied Energy, Elsevier, vol. 157(C), pages 546-553.
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    3. Zeng, Jimin & Xiao, Rui & Yuan, Jun, 2021. "High-quality syngas production from biomass driven by chemical looping on a PY-GA coupled reactor," Energy, Elsevier, vol. 214(C).
    4. Huang, Zhen & Deng, Zhengbing & Chen, Dezhen & He, Fang & Liu, Shuai & Zhao, Kun & Wei, Guoqiang & Zheng, Anqing & Zhao, Zengli & Li, Haibin, 2017. "Thermodynamic analysis and kinetic investigations on biomass char chemical looping gasification using Fe-Ni bimetallic oxygen carrier," Energy, Elsevier, vol. 141(C), pages 1836-1844.
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    Cited by:

    1. Chang, Yuxue & Li, Guang & Ma, Shuqi & Zhao, Xiaolei & Li, Na & Zhou, Xing & Zhang, Yulong, 2022. "Effect of hierarchical pore structure of oxygen carrier on the performance of biomass chemical looping hydrogen generation," Energy, Elsevier, vol. 254(PB).
    2. Wang, Xun & Fu, Genshen & Xiao, Bo & Xu, Tingting, 2022. "Optimization of nickel-iron bimetallic oxides for coproduction of hydrogen and syngas in chemical looping reforming with water splitting process," Energy, Elsevier, vol. 246(C).

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