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Effect of hierarchical pore structure of oxygen carrier on the performance of biomass chemical looping hydrogen generation

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  • Chang, Yuxue
  • Li, Guang
  • Ma, Shuqi
  • Zhao, Xiaolei
  • Li, Na
  • Zhou, Xing
  • Zhang, Yulong

Abstract

Biomass chemical looping hydrogen generation is known as a promising technique that converts biomass and water into hydrogen with inherent CO2 separation. In this study, effect of hierarchical pore structure of oxygen carrier on the performance of the biomass chemical looping hydrogen generation is investigated. The results show that oxygen carrier Fe2O3/Al2O3 with 0.09 g poly (ethylene oxide) can simultaneously improve the redox stability and activity. The hydrogen production of Fe2O3/Al2O3 with 0.09 g poly (ethylene oxide) and Fe2O3/Al2O3 without poly (ethylene oxide) are 343 ml H2/g oxygen carrier and 79 ml H2/g oxygen carrier, respectively. The above results are attributed to the hierarchical pore structure of the Fe2O3/Al2O3 with 0.09 g poly (ethylene oxide), which can create more active sites and prolong the contact time between the reactant and the oxygen carrier. Furthermore, the hierarchical pore structure of the oxygen carrier studied in this paper can be extended to design high active and stable oxygen carrier.

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  • Chang, Yuxue & Li, Guang & Ma, Shuqi & Zhao, Xiaolei & Li, Na & Zhou, Xing & Zhang, Yulong, 2022. "Effect of hierarchical pore structure of oxygen carrier on the performance of biomass chemical looping hydrogen generation," Energy, Elsevier, vol. 254(PB).
    • Handle: RePEc:eee:energy:v:254:y:2022:i:pb:s036054422201204x
    DOI: 10.1016/j.energy.2022.124301
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    References listed on IDEAS

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    1. Samprón, Iván & de Diego, Luis F. & García-Labiano, Francisco & Izquierdo, María T., 2021. "Optimization of synthesis gas production in the biomass chemical looping gasification process operating under auto-thermal conditions," Energy, Elsevier, vol. 226(C).
    2. Surywanshi, Gajanan Dattarao & Patnaikuni, Venkata Suresh & Vooradi, Ramsagar & Anne, Sarath Babu, 2021. "4-E and life cycle analyses of a supercritical coal direct chemical looping combustion power plant with hydrogen and power co-generation," Energy, Elsevier, vol. 217(C).
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    5. Li, Guang & Chang, Yuxue & Liu, Tao & Yu, Zhongliang & Liu, Zheyu & Liu, Fan & Ma, Shuqi & Weng, Yujing & Zhang, Yulong, 2020. "Hydrogen element flow and economic analyses of a coal direct chemical looping hydrogen generation process," Energy, Elsevier, vol. 206(C).
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    1. Quan, Jinxia & Miao, Zhenwu & Lin, Yousheng & Lv, Juan & Liu, Hailu & Feng, Chunzhou & Jiang, Enchen & Hu, Zhifeng, 2023. "Agglomeration mechanism of Fe2O3/Al2O3 oxygen carrier in chemical looping gasification," Energy, Elsevier, vol. 284(C).

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