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Efficient hydrogen production with CO2 capture using gas switching reforming

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  • Nazir, Shareq Mohd
  • Cloete, Jan Hendrik
  • Cloete, Schalk
  • Amini, Shahriar

Abstract

Hydrogen is a promising carbon-neutral energy carrier for a future decarbonized energy sector. This work presents process simulation studies of the gas switching reforming (GSR) process for hydrogen production with integrated CO2 capture (GSR-H2 process) at a minimal energy penalty. Like the conventional steam methane reforming (SMR) process, GSR combusts the off-gas fuel from the pressure swing adsorption unit to supply heat to the endothermic reforming reactions. However, GSR completes this combustion using the chemical looping combustion mechanism to achieve fuel combustion with CO2 separation. For this reason, the GSR-H2 plant incurred an energy penalty of only 3.8 %-points relative to the conventional SMR process with 96% CO2 capture. Further studies showed that the efficiency penalty is reduced to 0.3 %-points by including additional thermal mass in the reactor to maintain a higher reforming temperature, thereby facilitating a lower steam to carbon ratio. GSR reactors are standalone bubbling fluidized beds that will be relatively easy to scale up and operate under pressurized conditions, and the rest of the process layout uses commercially available technologies. The ability to produce clean hydrogen with no energy penalty combined with this inherent scalability makes the GSR-H2 plant a promising candidate for further research.

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  • Nazir, Shareq Mohd & Cloete, Jan Hendrik & Cloete, Schalk & Amini, Shahriar, 2019. "Efficient hydrogen production with CO2 capture using gas switching reforming," Energy, Elsevier, vol. 185(C), pages 372-385.
    • Handle: RePEc:eee:energy:v:185:y:2019:i:c:p:372-385
    DOI: 10.1016/j.energy.2019.07.072
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    1. Szima, Szabolcs & Nazir, Shareq Mohd & Cloete, Schalk & Amini, Shahriar & Fogarasi, Szabolcs & Cormos, Ana-Maria & Cormos, Calin-Cristian, 2019. "Gas switching reforming for flexible power and hydrogen production to balance variable renewables," Renewable and Sustainable Energy Reviews, Elsevier, vol. 110(C), pages 207-219.
    2. Nazir, Shareq Mohd & Cloete, Jan Hendrik & Cloete, Schalk & Amini, Shahriar, 2019. "Gas switching reforming (GSR) for power generation with CO2 capture: Process efficiency improvement studies," Energy, Elsevier, vol. 167(C), pages 757-765.
    3. Nikolaidis, Pavlos & Poullikkas, Andreas, 2017. "A comparative overview of hydrogen production processes," Renewable and Sustainable Energy Reviews, Elsevier, vol. 67(C), pages 597-611.
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    7. Carminati, Hudson Bolsoni & de Medeiros, José Luiz & Moure, Gustavo Torres & Barbosa, Lara Costa & Araújo, Ofélia de Queiroz F., 2020. "Low-emission pre-combustion gas-to-wire via ionic-liquid [Bmim][NTf2] absorption with high-pressure stripping," Renewable and Sustainable Energy Reviews, Elsevier, vol. 131(C).
    8. Zhang, Rui & Cao, Xuewen & Zhang, Xingwang & Yang, Jian & Bian, Jiang, 2024. "Co-benefits of the liquid hydrogen economy and LNG economy: Advances in LNG integrating LH2 production processes," Energy, Elsevier, vol. 301(C).
    9. Arnaiz del Pozo, Carlos & Cloete, Schalk & Jiménez Álvaro, Ángel, 2023. "Ammonia from solid fuels: A cost-effective route to energy security with negative CO2 emissions," Energy, Elsevier, vol. 278(PA).
    10. Cloete, Schalk & Hirth, Lion, 2020. "Flexible power and hydrogen production: Finding synergy between CCS and variable renewables," Energy, Elsevier, vol. 192(C).
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