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PVD synthesis of binder-free silicon and carbon coated 3D α-Fe2O3 nanorods hybrid films as high-capacity and long-life anode for flexible lithium-ion batteries

Author

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  • Wang, Mingyue
  • Huang, Ying
  • Wang, Ke
  • Zhu, Yade
  • Zhang, Na
  • Zhang, Hongming
  • Li, Suping
  • Feng, Zhenhe

Abstract

Flexible lithium-ion batteries are being given great attention as up-and-coming power source for the development of flexible and wearable electronic devices. In this work, a carbon and silicon coated 3D α-Fe2O3 nanorod arrays on carbon cloth composite was firstly designed by facile hydrothermal method and physical vapor deposition process. The as-prepared composite can be directly applied as flexible anode for Li-ion batteries without adding any binder and conducting materials. The electrochemical results show that the composite exhibits outstanding electrochemical lithium storage properties with high initial Coulombic Efficiency of 76% at 100 mA g−1 current density and a superior cycling performance that could maintain about 910 mAh·g−1 after 500 cycles at a 500 mA g−1 current density, which is two to three times of commercial graphite anodes. This study offers a promising route to greatly enhance the electrochemical properties of metal oxides and provides suggestive insights for developing high-performance electrode materials for flexible energy storage devices.

Suggested Citation

  • Wang, Mingyue & Huang, Ying & Wang, Ke & Zhu, Yade & Zhang, Na & Zhang, Hongming & Li, Suping & Feng, Zhenhe, 2018. "PVD synthesis of binder-free silicon and carbon coated 3D α-Fe2O3 nanorods hybrid films as high-capacity and long-life anode for flexible lithium-ion batteries," Energy, Elsevier, vol. 164(C), pages 1021-1029.
    • Handle: RePEc:eee:energy:v:164:y:2018:i:c:p:1021-1029
    DOI: 10.1016/j.energy.2018.09.046
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    2. Yang, Yang & Yuan, Wei & Zhang, Xiaoqing & Yuan, Yuhang & Wang, Chun & Ye, Yintong & Huang, Yao & Qiu, Zhiqiang & Tang, Yong, 2020. "Overview on the applications of three-dimensional printing for rechargeable lithium-ion batteries," Applied Energy, Elsevier, vol. 257(C).
    3. Tan Thong, Pham & Sadhasivam, T. & Kim, Nam-In & Kim, Yoong Ahm & Roh, Sung-Hee & Jung, Ho-Young, 2021. "Highly conductive current collector for enhancing conductivity and power supply of flexible thin-film Zn–MnO2 battery," Energy, Elsevier, vol. 221(C).

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