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Exploring particle-current collector contact damage in Li-ion battery using DEM-FEM scheme

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  • Song, Yanjie
  • Gao, Kai
  • He, Chunwang
  • Wu, Yikun
  • Yang, Shuangquan
  • Li, Na
  • Yang, Le
  • Mao, Yiqi
  • Song, Wei-Li
  • Chen, Haosen

Abstract

Calendering is an essential step in the manufacturing process of lithium-ion batteries. However, the intrusion of active particles into metal foil can damage the current collector during calendering. Here, we investigate the changes in surface morphology and the tensile properties of current collector after calendering. The damage mechanisms of tensile strength reduction for current collector due to compressive pressure are revealed by combining the calendering tests, tensile experiments, and simulations. Specifically, the DEM-FEM scheme is proposed, which combines the discrete element method (DEM) with the finite element method (FEM) to characterize the mechanical behavior of current collectors after the intrusion of active particles. The results show that the current collectors become more brittle and vulnerable with the increase of compressive pressure. Finally, the failure phase diagrams are presented during the winding and electrochemical processes. This study can reveal the failure behavior of current collectors and guides the electrode manufacturing optimization.

Suggested Citation

  • Song, Yanjie & Gao, Kai & He, Chunwang & Wu, Yikun & Yang, Shuangquan & Li, Na & Yang, Le & Mao, Yiqi & Song, Wei-Li & Chen, Haosen, 2023. "Exploring particle-current collector contact damage in Li-ion battery using DEM-FEM scheme," Applied Energy, Elsevier, vol. 351(C).
    • Handle: RePEc:eee:appene:v:351:y:2023:i:c:s0306261923012680
    DOI: 10.1016/j.apenergy.2023.121904
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    References listed on IDEAS

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    1. Jun Liu & Zhenan Bao & Yi Cui & Eric J. Dufek & John B. Goodenough & Peter Khalifah & Qiuyan Li & Bor Yann Liaw & Ping Liu & Arumugam Manthiram & Y. Shirley Meng & Venkat R. Subramanian & Michael F. T, 2019. "Pathways for practical high-energy long-cycling lithium metal batteries," Nature Energy, Nature, vol. 4(3), pages 180-186, March.
    2. Zhu, Juner & Zhang, Xiaowei & Luo, Hailing & Sahraei, Elham, 2018. "Investigation of the deformation mechanisms of lithium-ion battery components using in-situ micro tests," Applied Energy, Elsevier, vol. 224(C), pages 251-266.
    3. Yusheng Ye & Lien-Yang Chou & Yayuan Liu & Hansen Wang & Hiang Kwee Lee & Wenxiao Huang & Jiayu Wan & Kai Liu & Guangmin Zhou & Yufei Yang & Ankun Yang & Xin Xiao & Xin Gao & David Thomas Boyle & Hao , 2020. "Ultralight and fire-extinguishing current collectors for high-energy and high-safety lithium-ion batteries," Nature Energy, Nature, vol. 5(10), pages 786-793, October.
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