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The impedance of hydrogen oxidation reaction in a proton exchange membrane fuel cell in the presence of carbon monoxide in hydrogen stream

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  • Darowicki, K.
  • Gawel, L.
  • Mielniczek, M.
  • Zielinski, A.
  • Janicka, E.
  • Hunger, J.
  • Jorissen, L.

Abstract

Evaluation of performance of a proton exchange membrane fuel cell, which isaffected by carbon monoxide that pollutes the hydrogen stream, was presented. This influence was studied for carbon monoxide concentration of 125–325 ppb, which are close to values specified in ISO 14687:2019 standard. Performed studies provided crucial information for further development of fuel cell as an energy source for automotive application. Impedance with the use of Dynamic Electrochemical Impedance Spectroscopy profile measurements were completed for chosen carbon monoxide concentration under a constant current load andanode impedance variations were determined as a function of the time exposed to carbon monoxide. A method to determine the impedance of hydrogen oxidation was proposed. It was determined how the carbon monoxide surface coverage of anodic catalyst varies as a function of time. The capacitance of the double electrical layer and the charge transfer resistance of anodic reaction are discussed to evaluate them with respect to exposure time and surface coverage. It has been shown that proposed methodology can be used as a universal tool for testing fuel cells for both research and industrial applications, with the overall aim of optimization, monitoring, and diagnostics of the fuel cell.

Suggested Citation

  • Darowicki, K. & Gawel, L. & Mielniczek, M. & Zielinski, A. & Janicka, E. & Hunger, J. & Jorissen, L., 2020. "The impedance of hydrogen oxidation reaction in a proton exchange membrane fuel cell in the presence of carbon monoxide in hydrogen stream," Applied Energy, Elsevier, vol. 279(C).
    • Handle: RePEc:eee:appene:v:279:y:2020:i:c:s0306261920313404
    DOI: 10.1016/j.apenergy.2020.115868
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    References listed on IDEAS

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    Cited by:

    1. Li, Zheng & Wang, Yameng & Mu, Yongbiao & Wu, Buke & Jiang, Yuting & Zeng, Lin & Zhao, Tianshou, 2023. "Recent advances in the anode catalyst layer for proton exchange membrane fuel cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 176(C).
    2. Novella, Ricardo & García, Antonio & Gomez-Soriano, Josep & Fogué-Robles, Álvaro, 2023. "Exploring dilution potential for full load operation of medium duty hydrogen engine for the transport sector," Applied Energy, Elsevier, vol. 349(C).
    3. Perčić, Maja & Vladimir, Nikola & Jovanović, Ivana & Koričan, Marija, 2022. "Application of fuel cells with zero-carbon fuels in short-sea shipping," Applied Energy, Elsevier, vol. 309(C).
    4. Michal Mielniczek & Ewa Janicka & Lukasz Gawel & Kazimierz Darowicki, 2021. "Evaluation of Temperature Influence on Electrochemical Processes Occurring in a Lithium-Ion Supercapacitor with the Use of Dynamic Electrochemical Impedance Spectroscopy," Energies, MDPI, vol. 14(13), pages 1-12, June.

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