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80 Hours operation of a tubular solid oxide fuel cell using propane/air

Author

Listed:
  • Chen, Yu
  • Lu, Minyi
  • Yang, Huazheng
  • Yao, Yingbang
  • Tao, Tao
  • Lu, Shengguo
  • Wang, Chao
  • Ramesh, Rajendran
  • Kendall, Michaela
  • Kendall, Kevin
  • Ouyang, Xiaoping
  • Liang, Bo

Abstract

High power density and simple design are vital for these fuel cell-based portable power generation devices. This study provides an 8.6 g tubular SOFC with embedded a catalytic partial oxidation reformer, which is fabricated and operated for more than 100 h using propane/air. Nickel-iron nanosheets, as catalysts for reforming, supported on α-Al2O3 foam ceramic are synthesized by hydrothermal treatment. Testing for 80 h gives a power degradation of about 20% compared with the initial value. It is mainly attributed to sulfur-poisoning of nickel near anode/electrolyte interface according to transmission electron microscope (TEM) analysis. From TEM/energy dispersive spectroscopy line-scan results across the anode/electrolyte interface, sulfur as either aggregate at the nickel/yttria-stabilized zirconia grain boundaries or on the nickel grain surface, and no obvious carbon phase is founded. The maximum power density is 0.67 W cm−2 at 700 °C using propane/air (12 vol% propane), about 5% higher than the same cell using 20 vol% hydrogen.

Suggested Citation

  • Chen, Yu & Lu, Minyi & Yang, Huazheng & Yao, Yingbang & Tao, Tao & Lu, Shengguo & Wang, Chao & Ramesh, Rajendran & Kendall, Michaela & Kendall, Kevin & Ouyang, Xiaoping & Liang, Bo, 2020. "80 Hours operation of a tubular solid oxide fuel cell using propane/air," Applied Energy, Elsevier, vol. 272(C).
    • Handle: RePEc:eee:appene:v:272:y:2020:i:c:s0306261920306115
    DOI: 10.1016/j.apenergy.2020.115099
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    Cited by:

    1. Liang, Bo & Yao, Yue & Guo, Jin & Yang, Huazheng & Liang, Jiajiang & Zhao, Zhijiang & Wu, Gang & Zhan, Yuedong & Zhao, Xiaobo & Tao, Tao & Yao, Yingbang & Lu, Shengguo & Ruirui, Zhao, 2022. "Propane-fuelled microtubular solid oxide fuel cell stack electrically connected by an anodic rectangular window," Applied Energy, Elsevier, vol. 309(C).
    2. Wang, Chao & Liao, Mingzheng & Jiang, Zhiqiang & Liang, Bo & Weng, Jiahong & Song, Qingbin & Zhao, Ming & Chen, Ying & Lei, Libin, 2022. "Sorption-enhanced propane partial oxidation hydrogen production for solid oxide fuel cell (SOFC) applications," Energy, Elsevier, vol. 247(C).
    3. Wang, Jincheng & Zhao, Kai & Zhao, Jishi & Li, Jun & Liu, Yihui & Chen, Dongchu & Xu, Qing & Chen, Min, 2022. "A NiMo-YSZ catalyst support layer for regenerable solid oxide fuel cells running on isooctane," Applied Energy, Elsevier, vol. 326(C).
    4. Yao, Yue & Ma, Yue & Wang, Chenpeng & Ye, Hao & Liu, Yinglong & Liu, Jiawei & Zhao, Xiaobo & Tao, Tao & Yao, Yingbang & Lu, Shengguo & Yang, Huazheng & Liang, Bo, 2022. "A cofuel channel microtubular solid oxide fuel/electrolysis cell," Applied Energy, Elsevier, vol. 327(C).
    5. Dai, Huidong & Besser, R.S., 2022. "Understanding hydrogen sulfide impact on a portable, commercial, propane-powered solid-oxide fuel cell," Applied Energy, Elsevier, vol. 307(C).

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