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Advancement of ammonia based post-combustion CO2 capture using the advanced flash stripper process

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  • Jiang, Kaiqi
  • Li, Kangkang
  • Yu, Hai
  • Chen, Zuliang
  • Wardhaugh, Leigh
  • Feron, Paul

Abstract

The energy consumption associated with absorbent regeneration remains the most critical challenge for the industrial implementation of chemisorption based CO2 capture processes. Aimed at reducing the energy consumption, this paper proposes a promising process modification of the ammonia (NH3) based CO2 capture process that involves an advanced flash stripper with a cold rich split. We investigated the techno-economic performance of the advanced NH3 process integrated with a 650MW coal-fired power plant, and evaluated it technical and energy performance using a rigorous, rate-based model in Aspen Plus. A sensitivity study was also performed to optimise the modelling parameters, i.e. the stripper pressure and the absorbent NH3 concentration, and minimize the regeneration duty. A very competitive regeneration duty of 1.86MJ/kg CO2 was achieved for an optimised stripper pressure of 12bar and an NH3 concentration of 10.2 wt%, with a total equivalent work of 0.164MWh/t CO2 for absorbent pumping, NH3 regeneration and CO2 compression. We also used a validated economic model to estimate the capital investment of the advanced NH3 process and its corresponding economic performance. With its significant reduction in energy consumption, the proposed process was economically competitive with CO2 avoided cost was as low as US$40.7/t CO2. This was 34% and 44% less than the reference NH3 and monoethanolamine (MEA) processes, respectively. The advanced NH3 based flash stripper also had technical and economic advantages over other amine absorbents, such as MEA and piperazine (PZ), as well as other advanced stripper modifications, such as inter-heating process, revealing its process viability in commercial application.

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  • Jiang, Kaiqi & Li, Kangkang & Yu, Hai & Chen, Zuliang & Wardhaugh, Leigh & Feron, Paul, 2017. "Advancement of ammonia based post-combustion CO2 capture using the advanced flash stripper process," Applied Energy, Elsevier, vol. 202(C), pages 496-506.
    • Handle: RePEc:eee:appene:v:202:y:2017:i:c:p:496-506
    DOI: 10.1016/j.apenergy.2017.05.143
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    1. Li, Kangkang & Yu, Hai & Qi, Guojie & Feron, Paul & Tade, Moses & Yu, Jingwen & Wang, Shujuan, 2015. "Rate-based modelling of combined SO2 removal and NH3 recycling integrated with an aqueous NH3-based CO2 capture process," Applied Energy, Elsevier, vol. 148(C), pages 66-77.
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    1. Qi, Guojie & Wang, Shujuan, 2017. "Experimental study and rate-based modeling on combined CO2 and SO2 absorption using aqueous NH3 in packed column," Applied Energy, Elsevier, vol. 206(C), pages 1532-1543.
    2. Cheng, Chin-hung & Li, Kangkang & Yu, Hai & Jiang, Kaiqi & Chen, Jian & Feron, Paul, 2018. "Amine-based post-combustion CO2 capture mediated by metal ions: Advancement of CO2 desorption using copper ions," Applied Energy, Elsevier, vol. 211(C), pages 1030-1038.
    3. Jiang, Kaiqi & Yu, Hai & Chen, Linghong & Fang, Mengxiang & Azzi, Merched & Cottrell, Aaron & Li, Kangkang, 2020. "An advanced, ammonia-based combined NOx/SOx/CO2 emission control process towards a low-cost, clean coal technology," Applied Energy, Elsevier, vol. 260(C).
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    8. Song, Chunfeng & Liu, Qingling & Ji, Na & Deng, Shuai & Zhao, Jun & Kitamura, Yutaka, 2017. "Natural gas purification by heat pump assisted MEA absorption process," Applied Energy, Elsevier, vol. 204(C), pages 353-361.
    9. Muhammad Asif & Muhammad Suleman & Ihtishamul Haq & Syed Asad Jamal, 2018. "Post‐combustion CO2 capture with chemical absorption and hybrid system: current status and challenges," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 8(6), pages 998-1031, December.
    10. Rongrong Zhai & Hongtao Liu & Hao Wu & Hai Yu & Yongping Yang, 2018. "Analysis of Integration of MEA-Based CO 2 Capture and Solar Energy System for Coal-Based Power Plants Based on Thermo-Economic Structural Theory," Energies, MDPI, vol. 11(5), pages 1-30, May.
    11. Oh, Se-Young & Yun, Seokwon & Kim, Jin-Kuk, 2018. "Process integration and design for maximizing energy efficiency of a coal-fired power plant integrated with amine-based CO2 capture process," Applied Energy, Elsevier, vol. 216(C), pages 311-322.
    12. Liu, Sen & Gao, Hongxia & He, Chuan & Liang, Zhiwu, 2019. "Experimental evaluation of highly efficient primary and secondary amines with lower energy by a novel method for post-combustion CO2 capture," Applied Energy, Elsevier, vol. 233, pages 443-452.
    13. Liu, Fei & Fang, Mengxiang & Dong, Wenfeng & Wang, Tao & Xia, Zhixiang & Wang, Qinhui & Luo, Zhongyang, 2019. "Carbon dioxide absorption in aqueous alkanolamine blends for biphasic solvents screening and evaluation," Applied Energy, Elsevier, vol. 233, pages 468-477.
    14. Li, Kangkang & Jiang, Kaiqi & Jones, Timothy W. & Feron, Paul H.M. & Bennett, Robert D. & Hollenkamp, Anthony F., 2019. "CO2 regenerative battery for energy harvesting from ammonia-based post-combustion CO2 capture," Applied Energy, Elsevier, vol. 247(C), pages 417-425.
    15. Wang, Rujie & Liu, Shanshan & Wang, Lidong & Li, Qiangwei & Zhang, Shihan & Chen, Bo & Jiang, Lei & Zhang, Yifeng, 2019. "Superior energy-saving splitter in monoethanolamine-based biphasic solvents for CO2 capture from coal-fired flue gas," Applied Energy, Elsevier, vol. 242(C), pages 302-310.
    16. Zhang, Shihan & Shen, Yao & Wang, Lidong & Chen, Jianmeng & Lu, Yongqi, 2019. "Phase change solvents for post-combustion CO2 capture: Principle, advances, and challenges," Applied Energy, Elsevier, vol. 239(C), pages 876-897.
    17. Ji, Long & Yu, Hai & Li, Kangkang & Yu, Bing & Grigore, Mihaela & Yang, Qi & Wang, Xiaolong & Chen, Zuliang & Zeng, Ming & Zhao, Shuaifei, 2018. "Integrated absorption-mineralisation for low-energy CO2 capture and sequestration," Applied Energy, Elsevier, vol. 225(C), pages 356-366.
    18. Wang, Changhong & Jiang, Kaiqi & Yu, Hai & Yang, Shenghai & Li, Kangkang, 2022. "Copper electrowinning-coupled CO2 capture in solvent based post-combustion capture," Applied Energy, Elsevier, vol. 316(C).
    19. Madeddu, Claudio & Errico, Massimiliano & Baratti, Roberto, 2018. "Process analysis for the carbon dioxide chemical absorption–regeneration system," Applied Energy, Elsevier, vol. 215(C), pages 532-542.
    20. Oh, Hyun-Taek & Ju, Youngsan & Chung, Kyounghee & Lee, Chang-Ha, 2020. "Techno-economic analysis of advanced stripper configurations for post-combustion CO2 capture amine processes," Energy, Elsevier, vol. 206(C).
    21. Jiang, Kaiqi & Li, Kangkang, 2023. "Harvesting CO2 reaction enthalpy from amine scrubbing," Energy, Elsevier, vol. 284(C).
    22. Tamura, Masato & Gotou, Takahiro & Ishii, Hiroki & Riechelmann, Dirk, 2020. "Experimental investigation of ammonia combustion in a bench scale 1.2 MW-thermal pulverised coal firing furnace," Applied Energy, Elsevier, vol. 277(C).

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