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A mixed-pH dual-electrolyte microfluidic aluminum–air cell with high performance

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  • Chen, Binbin
  • Leung, Dennis Y.C.
  • Xuan, Jin
  • Wang, Huizhi

Abstract

Energy storage capacity has been a major limiting factor in pursuit of increasing functionality and mobility for portable devices. To increase capacity limits, novel battery designs with multi-electron redox couples and increased voltages have been listed as a priority research direction by the US Department of Energy. This study leverages the benefits of microfluidics technology to develop a novel mixed-pH media aluminum–air cell which incorporates the advantages of the trivalence of aluminum and mixed-pH thermodynamics. Experimentally, the new cell exhibited an open circuit potential of 2.2V and a maximum power density of 176mWcm−2, which are respectively 37.5% and 104.6% higher than conventional single alkaline aluminum–air cell under similar conditions. With further optimization of channel thickness, a power density of 216mWcm−2 was achieved in the present study.

Suggested Citation

  • Chen, Binbin & Leung, Dennis Y.C. & Xuan, Jin & Wang, Huizhi, 2017. "A mixed-pH dual-electrolyte microfluidic aluminum–air cell with high performance," Applied Energy, Elsevier, vol. 185(P2), pages 1303-1308.
    • Handle: RePEc:eee:appene:v:185:y:2017:i:p2:p:1303-1308
    DOI: 10.1016/j.apenergy.2015.10.029
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    References listed on IDEAS

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    1. Wang, Huizhi & Leung, Dennis Y.C. & Leung, Michael K.H., 2012. "Energy analysis of hydrogen and electricity production from aluminum-based processes," Applied Energy, Elsevier, vol. 90(1), pages 100-105.
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    4. Zhang, Hao & Xuan, Jin & Xu, Hong & Leung, Michael K.H. & Leung, Dennis Y.C. & Zhang, Li & Wang, Huizhi & Wang, Lei, 2013. "Enabling high-concentrated fuel operation of fuel cells with microfluidic principles: A feasibility study," Applied Energy, Elsevier, vol. 112(C), pages 1131-1137.
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    Cited by:

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    2. Samir De, Biswajit & Cunningham, Joshua & Khare, Neeraj & Luo, Jing-Li & Elias, Anastasia & Basu, Suddhasatwa, 2022. "Hydrogen generation and utilization in a two-phase flow membraneless microfluidic electrolyzer-fuel cell tandem operation for micropower application," Applied Energy, Elsevier, vol. 305(C).
    3. Ouyang, Tiancheng & Lu, Jie & Zhao, Zhongkai & Chen, Jingxian & Xu, Peihang, 2021. "New insight on the mechanism of vibration effects in vapor-feed microfluidic fuel cell," Energy, Elsevier, vol. 225(C).
    4. Tan, P. & Jiang, H.R. & Zhu, X.B. & An, L. & Jung, C.Y. & Wu, M.C. & Shi, L. & Shyy, W. & Zhao, T.S., 2017. "Advances and challenges in lithium-air batteries," Applied Energy, Elsevier, vol. 204(C), pages 780-806.
    5. Wang, Yifei & Kwok, Holly Y.H. & Pan, Wending & Zhang, Huimin & Lu, Xu & Leung, Dennis Y.C., 2019. "Parametric study and optimization of a low-cost paper-based Al-air battery with corrosion inhibition ability," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    6. Wei, Manhui & Wang, Keliang & Pei, Pucheng & Zhong, Liping & Züttel, Andreas & Pham, Thi Ha My & Shang, Nuo & Zuo, Yayu & Wang, Hengwei & Zhao, Siyuan, 2023. "Zinc carboxylate optimization strategy for extending Al-air battery system's lifetime," Applied Energy, Elsevier, vol. 350(C).
    7. Rewatkar, Prakash & Goel, Sanket, 2021. "Catalyst-mitigated arrayed aluminum-air origami fuel cell with ink-jet printed custom-porosity cathode," Energy, Elsevier, vol. 224(C).
    8. Feng, Shan & Yang, Guandong & Zheng, Dawei & Rauf, Abdur & Khan, Ubaid & Cheng, Rui & Wang, Lei & Wang, Wentao & Liu, Fude, 2022. "A high-performance tri-electrolyte aluminum-air microfluidic cell with a co-laminar-flow-and-bridging-electrolyte configuration," Applied Energy, Elsevier, vol. 307(C).

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