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Polar Bloch points in strained ferroelectric films

Author

Listed:
  • Yu-Jia Wang

    (Chinese Academy of Sciences)

  • Yan-Peng Feng

    (Songshan Lake Materials Laboratory
    Quantum Science Center of Guangdong-HongKong-Macau Greater Bay Area)

  • Yun-Long Tang

    (Chinese Academy of Sciences)

  • Yin-Lian Zhu

    (Songshan Lake Materials Laboratory
    Quantum Science Center of Guangdong-HongKong-Macau Greater Bay Area
    Hunan University of Science and Technology)

  • Yi Cao

    (Chinese Academy of Sciences
    University of Science and Technology of China)

  • Min-Jie Zou

    (Songshan Lake Materials Laboratory
    Quantum Science Center of Guangdong-HongKong-Macau Greater Bay Area)

  • Wan-Rong Geng

    (Songshan Lake Materials Laboratory
    Quantum Science Center of Guangdong-HongKong-Macau Greater Bay Area)

  • Xiu-Liang Ma

    (Songshan Lake Materials Laboratory
    Quantum Science Center of Guangdong-HongKong-Macau Greater Bay Area
    Chinese Academy of Sciences
    Lanzhou University of Technology)

Abstract

Topological domain structures have drawn great attention as they have potential applications in future electronic devices. As an important concept linking the quantum and classical magnetism, a magnetic Bloch point, predicted in 1960s but not observed directly so far, is a singular point around which magnetization vectors orient to nearly all directions. Here we show polar Bloch points in tensile-strained ultrathin ferroelectric PbTiO3 films, which are alternatively visualized by phase-field simulations and aberration-corrected scanning transmission electron microscopic imaging. The phase-field simulations indicate local steady-state negative capacitance around the Bloch points. The observation of polar Bloch points and their emergent properties consequently implies novel applications in future integrated circuits and low power electronic devices.

Suggested Citation

  • Yu-Jia Wang & Yan-Peng Feng & Yun-Long Tang & Yin-Lian Zhu & Yi Cao & Min-Jie Zou & Wan-Rong Geng & Xiu-Liang Ma, 2024. "Polar Bloch points in strained ferroelectric films," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-48216-1
    DOI: 10.1038/s41467-024-48216-1
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    References listed on IDEAS

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    1. U. K. Rößler & A. N. Bogdanov & C. Pfleiderer, 2006. "Spontaneous skyrmion ground states in magnetic metals," Nature, Nature, vol. 442(7104), pages 797-801, August.
    2. X. Z. Yu & W. Koshibae & Y. Tokunaga & K. Shibata & Y. Taguchi & N. Nagaosa & Y. Tokura, 2018. "Transformation between meron and skyrmion topological spin textures in a chiral magnet," Nature, Nature, vol. 564(7734), pages 95-98, December.
    3. A. K. Yadav & C. T. Nelson & S. L. Hsu & Z. Hong & J. D. Clarkson & C. M. Schlepütz & A. R. Damodaran & P. Shafer & E. Arenholz & L. R. Dedon & D. Chen & A. Vishwanath & A. M. Minor & L. Q. Chen & J. , 2016. "Observation of polar vortices in oxide superlattices," Nature, Nature, vol. 530(7589), pages 198-201, February.
    4. A. K. Yadav & C. T. Nelson & S. L. Hsu & Z. Hong & J. D. Clarkson & C. M. Schlepütz & A. R. Damodaran & P. Shafer & E. Arenholz & L. R. Dedon & D. Chen & A. Vishwanath & A. M. Minor & L. Q. Chen & J. , 2016. "Correction: Corrigendum: Observation of polar vortices in oxide superlattices," Nature, Nature, vol. 534(7605), pages 138-138, June.
    5. Ajay K. Yadav & Kayla X. Nguyen & Zijian Hong & Pablo García-Fernández & Pablo Aguado-Puente & Christopher T. Nelson & Sujit Das & Bhagwati Prasad & Daewoong Kwon & Suraj Cheema & Asif I. Khan & Chenm, 2019. "Spatially resolved steady-state negative capacitance," Nature, Nature, vol. 565(7740), pages 468-471, January.
    6. Claire Donnelly & Manuel Guizar-Sicairos & Valerio Scagnoli & Sebastian Gliga & Mirko Holler & Jörg Raabe & Laura J. Heyderman, 2017. "Three-dimensional magnetization structures revealed with X-ray vector nanotomography," Nature, Nature, vol. 547(7663), pages 328-331, July.
    7. X. Z. Yu & Y. Onose & N. Kanazawa & J. H. Park & J. H. Han & Y. Matsui & N. Nagaosa & Y. Tokura, 2010. "Real-space observation of a two-dimensional skyrmion crystal," Nature, Nature, vol. 465(7300), pages 901-904, June.
    8. Mi-Young Im & Hee-Sung Han & Min-Seung Jung & Young-Sang Yu & Sooseok Lee & Seongsoo Yoon & Weilun Chao & Peter Fischer & Jung-Il Hong & Ki-Suk Lee, 2019. "Dynamics of the Bloch point in an asymmetric permalloy disk," Nature Communications, Nature, vol. 10(1), pages 1-8, December.
    9. S. Das & Y. L. Tang & Z. Hong & M. A. P. Gonçalves & M. R. McCarter & C. Klewe & K. X. Nguyen & F. Gómez-Ortiz & P. Shafer & E. Arenholz & V. A. Stoica & S.-L. Hsu & B. Wang & C. Ophus & J. F. Liu & C, 2019. "Observation of room-temperature polar skyrmions," Nature, Nature, vol. 568(7752), pages 368-372, April.
    10. Ajay K. Yadav & Kayla X. Nguyen & Zijian Hong & Pablo García-Fernández & Pablo Aguado-Puente & Christopher T. Nelson & Sujit Das & Bhagwati Prasad & Daewoong Kwon & Suraj Cheema & Asif I. Khan & Chenm, 2019. "Author Correction: Spatially resolved steady-state negative capacitance," Nature, Nature, vol. 568(7753), pages 13-13, April.
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