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Field-induced partial disorder in a Shastry-Sutherland lattice

Author

Listed:
  • Madalynn Marshall

    (Oak Ridge National Laboratory)

  • Brianna R. Billingsley

    (University of Arizona)

  • Xiaojian Bai

    (Oak Ridge National Laboratory
    University of Louisiana)

  • Qianli Ma

    (Oak Ridge National Laboratory)

  • Tai Kong

    (University of Arizona
    University of Arizona)

  • Huibo Cao

    (Oak Ridge National Laboratory)

Abstract

A 2-Q antiferromagnetic order of the ferromagnetic dimers was found below TN = 2.9 K in the Shastry-Sutherland lattice BaNd2ZnS5 by single crystal neutron diffraction. The magnetic order can be understood by the orthogonal arrangement of local Ising Nd spins, identified by polarized neutrons. A field was applied along [1 -1 0] to probe the observed metamagnetic transition in the magnetization measurement. The field decouples two magnetic sublattices corresponding to the propagation vectors q1 = (½, ½, 0) and q2 = (−½, ½, 0), respectively. Each sublattice shows a “stripe” order with a Néel-type arrangement in each single layer. The “stripe” order with q1 remains nearly intact up to 6 T, while the other one with q2 is suppressed at a critical field Hc ~1.7 T, indicating a partial disorder. The Hc varies with temperature and is manifested in the H-T phase diagram constructed by measuring the magnetization in BaNd2ZnS5.

Suggested Citation

  • Madalynn Marshall & Brianna R. Billingsley & Xiaojian Bai & Qianli Ma & Tai Kong & Huibo Cao, 2023. "Field-induced partial disorder in a Shastry-Sutherland lattice," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-39409-1
    DOI: 10.1038/s41467-023-39409-1
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    References listed on IDEAS

    as
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