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Continuous control of classical-quantum crossover by external high pressure in the coupled chain compound CsCuCl3

Author

Listed:
  • Daisuke Yamamoto

    (Nihon University
    Aoyama Gakuin University)

  • Takahiro Sakurai

    (Kobe University)

  • Ryosuke Okuto

    (Kobe University)

  • Susumu Okubo

    (Kobe University)

  • Hitoshi Ohta

    (Kobe University)

  • Hidekazu Tanaka

    (Tokyo Institute of Technology)

  • Yoshiya Uwatoko

    (The University of Tokyo)

Abstract

In solid materials, the parameters relevant to quantum effects, such as the spin quantum number, are basically determined and fixed at the chemical synthesis, which makes it challenging to control the amount of quantum correlations. We propose and demonstrate a method for active control of the classical-quantum crossover in magnetic insulators by applying external pressure. As a concrete example, we perform high-field, high-pressure measurements on CsCuCl3, which has the structure of weakly-coupled spin chains. The magnetization process experiences a continuous evolution from the semi-classical realm to the highly-quantum regime with increasing pressure. Based on the idea of "squashing” the spin chains onto a plane, we characterize the change in the quantum correlations by the change in the value of the local spin quantum number of an effective two-dimensional model. This opens a way to access the tunable classical-quantum crossover of two-dimensional spin systems by using alternative systems of coupled-chain compounds.

Suggested Citation

  • Daisuke Yamamoto & Takahiro Sakurai & Ryosuke Okuto & Susumu Okubo & Hitoshi Ohta & Hidekazu Tanaka & Yoshiya Uwatoko, 2021. "Continuous control of classical-quantum crossover by external high pressure in the coupled chain compound CsCuCl3," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-24542-6
    DOI: 10.1038/s41467-021-24542-6
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    References listed on IDEAS

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    1. Elliot Snider & Nathan Dasenbrock-Gammon & Raymond McBride & Mathew Debessai & Hiranya Vindana & Kevin Vencatasamy & Keith V. Lawler & Ashkan Salamat & Ranga P. Dias, 2020. "RETRACTED ARTICLE: Room-temperature superconductivity in a carbonaceous sulfur hydride," Nature, Nature, vol. 586(7829), pages 373-377, October.
    2. Leon Balents, 2010. "Spin liquids in frustrated magnets," Nature, Nature, vol. 464(7286), pages 199-208, March.
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