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Magnetically assisted drop-on-demand 3D printing of microstructured multimaterial composites

Author

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  • Wing Chung Liu

    (Nanyang Technological University)

  • Vanessa Hui Yin Chou

    (Nanyang Technological University)

  • Rohit Pratyush Behera

    (Nanyang Technological University)

  • Hortense Le Ferrand

    (Nanyang Technological University
    Nanyang Technological University)

Abstract

Microstructured composites with hierarchically arranged fillers fabricated by three-dimensional (3D) printing show enhanced properties along the fillers’ alignment direction. However, it is still challenging to achieve good control of the filler arrangement and high filler concentration simultaneously, which limits the printed material’s properties. In this study, we develop a magnetically assisted drop-on-demand 3D printing technique (MDOD) to print aligned microplatelet reinforced composites. By performing drop-on-demand printing using aqueous slurry inks while applying an external magnetic field, MDOD can print composites with microplatelet fillers aligned at set angles with high filler concentrations up to 50 vol%. Moreover, MDOD allows multimaterial printing with voxelated control. We showcase the capabilities of MDOD by printing multimaterial piezoresistive sensors with tunable performances based on the local microstructure and composition. MDOD thus creates a large design space to enhance the mechanical and functional properties of 3D printed electronic or sensing devices using a wide range of materials.

Suggested Citation

  • Wing Chung Liu & Vanessa Hui Yin Chou & Rohit Pratyush Behera & Hortense Le Ferrand, 2022. "Magnetically assisted drop-on-demand 3D printing of microstructured multimaterial composites," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32792-1
    DOI: 10.1038/s41467-022-32792-1
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    References listed on IDEAS

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    1. Dimitri Kokkinis & Manuel Schaffner & André R. Studart, 2015. "Multimaterial magnetically assisted 3D printing of composite materials," Nature Communications, Nature, vol. 6(1), pages 1-10, December.
    2. Robert D. Deegan & Olgica Bakajin & Todd F. Dupont & Greb Huber & Sidney R. Nagel & Thomas A. Witten, 1997. "Capillary flow as the cause of ring stains from dried liquid drops," Nature, Nature, vol. 389(6653), pages 827-829, October.
    3. Joshua J. Martin & Brad E. Fiore & Randall M. Erb, 2015. "Designing bioinspired composite reinforcement architectures via 3D magnetic printing," Nature Communications, Nature, vol. 6(1), pages 1-7, December.
    4. Cenxiao Tan & Zhigang Dong & Yehua Li & Haiguang Zhao & Xingyi Huang & Zhaocai Zhou & Jin-Wu Jiang & Yun-Ze Long & Pingkai Jiang & Tong-Yi Zhang & Bin Sun, 2020. "A high performance wearable strain sensor with advanced thermal management for motion monitoring," Nature Communications, Nature, vol. 11(1), pages 1-10, December.
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    1. Huawei Qu & Chongjian Gao & Kaizheng Liu & Hongya Fu & Zhiyuan Liu & Paul H. J. Kouwer & Zhenyu Han & Changshun Ruan, 2024. "Gradient matters via filament diameter-adjustable 3D printing," Nature Communications, Nature, vol. 15(1), pages 1-13, December.

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