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Programming crack patterns with light in colloidal plasmonic films

Author

Listed:
  • Fanny Thorimbert

    (Sorbonne Université, CNRS, UMR 7574, Chimie de la Matière Condensée de Paris)

  • Mateusz Odziomek

    (Max Planck Institute of Colloids and Interfaces)

  • Denis Chateau

    (Université Claude Bernard Lyon 1, Laboratoire de Chimie)

  • Stéphane Parola

    (Université Claude Bernard Lyon 1, Laboratoire de Chimie)

  • Marco Faustini

    (Sorbonne Université, CNRS, UMR 7574, Chimie de la Matière Condensée de Paris
    Institut Universitaire de France)

Abstract

Crack formation observed across diverse fields like geology, nanotechnology, arts, structural engineering or surface science, is a chaotic and undesirable phenomenon, resulting in random patterns of cracks generally leading to material failure. Limiting the formation of cracks or “programming” the path of cracks is a great technological challenge since it holds promise to enhance material durability or even to develop low cost patterning methods. Drawing inspiration from negative phototropism in plants, we demonstrate the capability to organize, guide, replicate, or arrest crack propagation in colloidal films through remote light manipulation. The key consists in using plasmonic photothermal absorbers to generate “virtual” defects enabling controlled deviation of cracks. We engineer a dip-coating process coupled with selective light irradiation enabling simultaneous deposition and light-directed crack patterning. This approach represents a rare example of a robust self-assembly process with long-range order that can be programmed in both space and time.

Suggested Citation

  • Fanny Thorimbert & Mateusz Odziomek & Denis Chateau & Stéphane Parola & Marco Faustini, 2024. "Programming crack patterns with light in colloidal plasmonic films," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-45365-1
    DOI: 10.1038/s41467-024-45365-1
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    References listed on IDEAS

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    1. António F. Martins & Nigel C. Bennett & Sylvie Clavel & Herman Groenewald & Sean Hensman & Stefan Hoby & Antoine Joris & Paul R. Manger & Michel C. Milinkovitch, 2018. "Locally-curved geometry generates bending cracks in the African elephant skin," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
    2. Koo Hyun Nam & Il H. Park & Seung Hwan Ko, 2012. "Patterning by controlled cracking," Nature, Nature, vol. 485(7397), pages 221-224, May.
    3. Robert D. Deegan & Olgica Bakajin & Todd F. Dupont & Greb Huber & Sidney R. Nagel & Thomas A. Witten, 1997. "Capillary flow as the cause of ring stains from dried liquid drops," Nature, Nature, vol. 389(6653), pages 827-829, October.
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