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Catalytic production of low-carbon footprint sustainable natural gas

Author

Listed:
  • Xiaoqin Si

    (Chinese Academy of Sciences)

  • Rui Lu

    (Chinese Academy of Sciences)

  • Zhitong Zhao

    (Chinese Academy of Sciences)

  • Xiaofeng Yang

    (Chinese Academy of Sciences)

  • Feng Wang

    (Chinese Academy of Sciences)

  • Huifang Jiang

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Xiaolin Luo

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Aiqin Wang

    (Chinese Academy of Sciences)

  • Zhaochi Feng

    (Chinese Academy of Sciences)

  • Jie Xu

    (Chinese Academy of Sciences)

  • Fang Lu

    (Chinese Academy of Sciences)

Abstract

Natural gas is one of the foremost basic energy sources on earth. Although biological process appears as promising valorization routes to transfer biomass to sustainable methane, the recalcitrance of lignocellulosic biomass is the major limitation for the production of mixing gas to meet the natural gas composition of pipeline transportation. Here we develop a catalytic-drive approach to directly transfer solid biomass to bio-natural gas which can be suitable for the current infrastructure. A catalyst with Ni2Al3 alloy phase enables nearly complete conversion of various agricultural and forestry residues, the total carbon yield of gas products reaches up to 93% after several hours at relative low-temperature (300 degrees Celsius). And the catalyst shows powerful processing capability for the production of natural gas during thirty cycles. A low-carbon footprint is estimated by a preliminary life cycle assessment, especially for the low hydrogen pressure and non-fossil hydrogen, and technical economic analysis predicts that this process is an economically competitive production process.

Suggested Citation

  • Xiaoqin Si & Rui Lu & Zhitong Zhao & Xiaofeng Yang & Feng Wang & Huifang Jiang & Xiaolin Luo & Aiqin Wang & Zhaochi Feng & Jie Xu & Fang Lu, 2022. "Catalytic production of low-carbon footprint sustainable natural gas," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-021-27919-9
    DOI: 10.1038/s41467-021-27919-9
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    References listed on IDEAS

    as
    1. M. S. Dresselhaus & I. L. Thomas, 2001. "Alternative energy technologies," Nature, Nature, vol. 414(6861), pages 332-337, November.
    2. Qineng Xia & Zongjia Chen & Yi Shao & Xueqing Gong & Haifeng Wang & Xiaohui Liu & Stewart F. Parker & Xue Han & Sihai Yang & Yanqin Wang, 2016. "Direct hydrodeoxygenation of raw woody biomass into liquid alkanes," Nature Communications, Nature, vol. 7(1), pages 1-10, September.
    3. Devon Rowe & Atis Muehlenbachs, 1999. "Low-temperature thermal generation of hydrocarbon gases in shallow shales," Nature, Nature, vol. 398(6722), pages 61-63, March.
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    Cited by:

    1. Wang, Jia & Wen, Mengyuan & Ren, Jurong & La, Xinru & Meng, Xianzhi & Yuan, Xiangzhou & Ragauskas, Arthur J. & Jiang, Jianchun, 2024. "Tailoring microwave frequencies for high-efficiency hydrogen production from biomass," Energy, Elsevier, vol. 297(C).
    2. Wang, Jia & Jiang, Jianchun & Li, Dongxian & Meng, Xianzhi & Zhan, Guowu & Wang, Yunpu & Zhang, Aihua & Sun, Yunjuan & Ruan, Roger & Ragauskas, Arthur J., 2022. "Creating values from wastes: Producing biofuels from waste cooking oil via a tandem vapor-phase hydrotreating process," Applied Energy, Elsevier, vol. 323(C).

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