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The future of low-temperature carbon dioxide electrolysis depends on solving one basic problem

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  • Joshua A. Rabinowitz

    (Stanford University)

  • Matthew W. Kanan

    (Stanford University)

Abstract

Carbonate formation is the primary source of energy and carbon losses in low-temperature carbon dioxide electrolysis. Realigning research priorities to address the carbonate problem is essential if this technology is to become a viable option for renewable chemical and fuel production.

Suggested Citation

  • Joshua A. Rabinowitz & Matthew W. Kanan, 2020. "The future of low-temperature carbon dioxide electrolysis depends on solving one basic problem," Nature Communications, Nature, vol. 11(1), pages 1-3, December.
    • Handle: RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-020-19135-8
    DOI: 10.1038/s41467-020-19135-8
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    Cited by:

    1. Ke Xie & Adnan Ozden & Rui Kai Miao & Yuhang Li & David Sinton & Edward H. Sargent, 2022. "Eliminating the need for anodic gas separation in CO2 electroreduction systems via liquid-to-liquid anodic upgrading," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    2. Mengran Li & Eric W. Lees & Wen Ju & Siddhartha Subramanian & Kailun Yang & Justin C. Bui & Hugo-Pieter Iglesias van Montfort & Maryam Abdinejad & Joost Middelkoop & Peter Strasser & Adam Z. Weber & A, 2024. "Local ionic transport enables selective PGM-free bipolar membrane electrode assembly," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    3. Hugo-Pieter Iglesias van Montfort & Mengran Li & Erdem Irtem & Maryam Abdinejad & Yuming Wu & Santosh K. Pal & Mark Sassenburg & Davide Ripepi & Siddhartha Subramanian & Jasper Biemolt & Thomas E. Ruf, 2023. "Non-invasive current collectors for improved current-density distribution during CO2 electrolysis on super-hydrophobic electrodes," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    4. Haifeng Shen & Huanyu Jin & Haobo Li & Herui Wang & Jingjing Duan & Yan Jiao & Shi-Zhang Qiao, 2023. "Acidic CO2-to-HCOOH electrolysis with industrial-level current on phase engineered tin sulfide," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    5. Xueping Qin & Heine A. Hansen & Karoliina Honkala & Marko M. Melander, 2023. "Cation-induced changes in the inner- and outer-sphere mechanisms of electrocatalytic CO2 reduction," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    6. Erfan Shirzadi & Qiu Jin & Ali Shayesteh Zeraati & Roham Dorakhan & Tiago J. Goncalves & Jehad Abed & Byoung-Hoon Lee & Armin Sedighian Rasouli & Joshua Wicks & Jinqiang Zhang & Pengfei Ou & Victor Bo, 2024. "Ligand-modified nanoparticle surfaces influence CO electroreduction selectivity," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    7. Mengran Li & Erdem Irtem & Hugo-Pieter Iglesias van Montfort & Maryam Abdinejad & Thomas Burdyny, 2022. "Energy comparison of sequential and integrated CO2 capture and electrochemical conversion," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    8. Jing Li & Haocheng Xiong & Xiaozhi Liu & Donghuan Wu & Dong Su & Bingjun Xu & Qi Lu, 2023. "Weak CO binding sites induced by Cu–Ag interfaces promote CO electroreduction to multi-carbon liquid products," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    9. Agnes E. Thorarinsdottir & Samuel S. Veroneau & Daniel G. Nocera, 2022. "Self-healing oxygen evolution catalysts," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    10. Kezia Megagita Gerby Langie & Kyungjae Tak & Changsoo Kim & Hee Won Lee & Kwangho Park & Dongjin Kim & Wonsang Jung & Chan Woo Lee & Hyung-Suk Oh & Dong Ki Lee & Jai Hyun Koh & Byoung Koun Min & Da Hy, 2022. "Toward economical application of carbon capture and utilization technology with near-zero carbon emission," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    11. Hai-Gang Qin & Yun-Fan Du & Yi-Yang Bai & Fu-Zhi Li & Xian Yue & Hao Wang & Jian-Zhao Peng & Jun Gu, 2023. "Surface-immobilized cross-linked cationic polyelectrolyte enables CO2 reduction with metal cation-free acidic electrolyte," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    12. Bin Liu & Tuo Wang & Shujie Wang & Gong Zhang & Dazhong Zhong & Tenghui Yuan & Hao Dong & Bo Wu & Jinlong Gong, 2022. "Back-illuminated photoelectrochemical flow cell for efficient CO2 reduction," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    13. Ke Xie & Rui Kai Miao & Adnan Ozden & Shijie Liu & Zhu Chen & Cao-Thang Dinh & Jianan Erick Huang & Qiucheng Xu & Christine M. Gabardo & Geonhui Lee & Jonathan P. Edwards & Colin P. O’Brien & Shannon , 2022. "Bipolar membrane electrolyzers enable high single-pass CO2 electroreduction to multicarbon products," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    14. Cornelius A. Obasanjo & Guorui Gao & Jackson Crane & Viktoria Golovanova & F. Pelayo García de Arquer & Cao-Thang Dinh, 2023. "High-rate and selective conversion of CO2 from aqueous solutions to hydrocarbons," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    15. Huiying Deng & Tingting Liu & Wenshan Zhao & Jundong Wang & Yuesheng Zhang & Shuzhen Zhang & Yu Yang & Chao Yang & Wenzhi Teng & Zhuo Chen & Gengfeng Zheng & Fengwang Li & Yaqiong Su & Jingshu Hui & Y, 2024. "Substituent tuning of Cu coordination polymers enables carbon-efficient CO2 electroreduction to multi-carbon products," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    16. Shoujie Li & Wei Chen & Xiao Dong & Chang Zhu & Aohui Chen & Yanfang Song & Guihua Li & Wei Wei & Yuhan Sun, 2022. "Hierarchical micro/nanostructured silver hollow fiber boosts electroreduction of carbon dioxide," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    17. Shoujie Li & Xiao Dong & Gangfeng Wu & Yanfang Song & Jianing Mao & Aohui Chen & Chang Zhu & Guihua Li & Yiheng Wei & Xiaohu Liu & Jiangjiang Wang & Wei Chen & Wei Wei, 2024. "Ampere-level CO2 electroreduction with single-pass conversion exceeding 85% in acid over silver penetration electrodes," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    18. Fiammetta Rita Bianchi & Barbara Bosio, 2021. "Operating Principles, Performance and Technology Readiness Level of Reversible Solid Oxide Cells," Sustainability, MDPI, vol. 13(9), pages 1-23, April.
    19. Yurou Celine Xiao & Siyu Sonia Sun & Yong Zhao & Rui Kai Miao & Mengyang Fan & Geonhui Lee & Yuanjun Chen & Christine M. Gabardo & Yan Yu & Chenyue Qiu & Zunmin Guo & Xinyue Wang & Panagiotis Papangel, 2024. "Reactive capture of CO2 via amino acid," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    20. Xiaojie She & Lingling Zhai & Yifei Wang & Pei Xiong & Molly Meng-Jung Li & Tai-Sing Wu & Man Chung Wong & Xuyun Guo & Zhihang Xu & Huaming Li & Hui Xu & Ye Zhu & Shik Chi Edman Tsang & Shu Ping Lau, 2024. "Pure-water-fed, electrocatalytic CO2 reduction to ethylene beyond 1,000 h stability at 10 A," Nature Energy, Nature, vol. 9(1), pages 81-91, January.
    21. Shashwati C. Cunha & Joaquin Resasco, 2023. "Maximizing single-pass conversion does not result in practical readiness for CO2 reduction electrolyzers," Nature Communications, Nature, vol. 14(1), pages 1-6, December.

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