Selective and stable CO2 electroreduction at high rates via control of local H2O/CO2 ratio
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DOI: 10.1038/s41467-024-50269-1
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- Chen Peng & Gan Luo & Junbo Zhang & Menghuan Chen & Zhiqiang Wang & Tsun-Kong Sham & Lijuan Zhang & Yafei Li & Gengfeng Zheng, 2021. "Double sulfur vacancies by lithium tuning enhance CO2 electroreduction to n-propanol," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
- Miao Zhong & Kevin Tran & Yimeng Min & Chuanhao Wang & Ziyun Wang & Cao-Thang Dinh & Phil De Luna & Zongqian Yu & Armin Sedighian Rasouli & Peter Brodersen & Song Sun & Oleksandr Voznyy & Chih-Shan Ta, 2020. "Accelerated discovery of CO2 electrocatalysts using active machine learning," Nature, Nature, vol. 581(7807), pages 178-183, May.
- Chanyeon Kim & Justin C. Bui & Xiaoyan Luo & Jason K. Cooper & Ahmet Kusoglu & Adam Z. Weber & Alexis T. Bell, 2021. "Tailored catalyst microenvironments for CO2 electroreduction to multicarbon products on copper using bilayer ionomer coatings," Nature Energy, Nature, vol. 6(11), pages 1026-1034, November.
- Carina Yi Jing Lim & Meltem Yilmaz & Juan Manuel Arce-Ramos & Albertus D. Handoko & Wei Jie Teh & Yuangang Zheng & Zi Hui Jonathan Khoo & Ming Lin & Mark Isaacs & Teck Lip Dexter Tam & Yang Bai & Chee, 2023. "Author Correction: Surface charge as activity descriptors for electrochemical CO2 reduction to multi-carbon products on organic-functionalised Cu," Nature Communications, Nature, vol. 14(1), pages 1-1, December.
- Adnan Ozden & Jun Li & Sharath Kandambeth & Xiao-Yan Li & Shijie Liu & Osama Shekhah & Pengfei Ou & Y. Zou Finfrock & Ya-Kun Wang & Tartela Alkayyali & F. Pelayo García de Arquer & Vinayak S. Kale & P, 2023. "Energy- and carbon-efficient CO2/CO electrolysis to multicarbon products via asymmetric ion migration–adsorption," Nature Energy, Nature, vol. 8(2), pages 179-190, February.
- Huali Wu & Ji Li & Kun Qi & Yang Zhang & Eddy Petit & Wensen Wang & Valérie Flaud & Nicolas Onofrio & Bertrand Rebiere & Lingqi Huang & Chrystelle Salameh & Luc Lajaunie & Philippe Miele & Damien Voir, 2021. "Improved electrochemical conversion of CO2 to multicarbon products by using molecular doping," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
- Jun Li & Adnan Ozden & Mingyu Wan & Yongfeng Hu & Fengwang Li & Yuhang Wang & Reza R. Zamani & Dan Ren & Ziyun Wang & Yi Xu & Dae-Hyun Nam & Joshua Wicks & Bin Chen & Xue Wang & Mingchuan Luo & Michae, 2021. "Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
- Dan Ren & Jinhuan Fong & Boon Siang Yeo, 2018. "The effects of currents and potentials on the selectivities of copper toward carbon dioxide electroreduction," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
- Zhuo Xing & Lin Hu & Donald S. Ripatti & Xun Hu & Xiaofeng Feng, 2021. "Enhancing carbon dioxide gas-diffusion electrolysis by creating a hydrophobic catalyst microenvironment," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
- Haeun Shin & Kentaro U. Hansen & Feng Jiao, 2021. "Techno-economic assessment of low-temperature carbon dioxide electrolysis," Nature Sustainability, Nature, vol. 4(10), pages 911-919, October.
- Joshua A. Rabinowitz & Matthew W. Kanan, 2020. "The future of low-temperature carbon dioxide electrolysis depends on solving one basic problem," Nature Communications, Nature, vol. 11(1), pages 1-3, December.
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