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Analysis of Perovskite Solar Cell Degradation over Time Using NIR Spectroscopy—A Novel Approach

Author

Listed:
  • Marek Gąsiorowski

    (Faculty of Electronics and Computer Science, Koszalin University of Technology, 75-453 Koszalin, Poland)

  • Shyantan Dasgupta

    (Faculty of Materials Engineering and Technical Physics, Poznan University of Technology, Piotrowo 3, 60-965 Poznan, Poland
    Saule Research Institute, Wroclaw Technology Park, 54-130 Wroclaw, Poland)

  • Leszek Bychto

    (Faculty of Electronics and Computer Science, Koszalin University of Technology, 75-453 Koszalin, Poland)

  • Taimoor Ahmad

    (Department of Physical Science and Engineering, King Abdullah University of Science and Technology, Thuwal 23955-6900, Saudi Arabia
    Saule Technologies, Wroclaw Technology Park, 54-130 Wroclaw, Poland)

  • Piotr Szymak

    (Faculty of Mechanical and Electrical Engineering, Polish Naval Academy, 81-127 Gdynia, Poland)

  • Konrad Wojciechowski

    (Saule Research Institute, Wroclaw Technology Park, 54-130 Wroclaw, Poland
    Saule Technologies, Wroclaw Technology Park, 54-130 Wroclaw, Poland)

  • Aleksy Patryn

    (Faculty of Electronics and Computer Science, Koszalin University of Technology, 75-453 Koszalin, Poland)

Abstract

In recent years, there has been a dynamic development of photovoltaic materials based on perovskite structures. Solar cells based on perovskite materials are characterised by a relatively high price/performance ratio. Achieving stability at elevated temperatures has remained one of the greatest challenges in the perovskite solar cell research community. However, significant progress in this field has been made by utilising different compositional engineering routes for the fabrication of perovskite semiconductors such as triple cation-based perovskite structures. In this work, a new approach for the rapid analysis of the changes occurring in time in perovskite structures was developed. We implemented a quick and inexpensive method of estimating the ageing of perovskite structures based on an express diagnosis of light reflection in the near-infrared region. The possibility of using optical reflectance in the NIR range (900–1700 nm) to observe the ageing of perovskite structures over time was investigated, and changes in optical reflectance spectra of original perovskite solar cell structures during one month after PSC production were monitored. The ratio of characteristic pikes in the reflection spectra was determined, and statistical analysis by the two-dimensional correlation spectroscopy (2D-COS) method was performed. This method allowed correctly detecting critical points in thermal ageing over time.

Suggested Citation

  • Marek Gąsiorowski & Shyantan Dasgupta & Leszek Bychto & Taimoor Ahmad & Piotr Szymak & Konrad Wojciechowski & Aleksy Patryn, 2022. "Analysis of Perovskite Solar Cell Degradation over Time Using NIR Spectroscopy—A Novel Approach," Energies, MDPI, vol. 15(15), pages 1-11, July.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:15:p:5397-:d:872101
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    1. Jaeki Jeong & Minjin Kim & Jongdeuk Seo & Haizhou Lu & Paramvir Ahlawat & Aditya Mishra & Yingguo Yang & Michael A. Hope & Felix T. Eickemeyer & Maengsuk Kim & Yung Jin Yoon & In Woo Choi & Barbara Pr, 2021. "Pseudo-halide anion engineering for α-FAPbI3 perovskite solar cells," Nature, Nature, vol. 592(7854), pages 381-385, April.
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