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Monolithic Perovskite/Silicon-Heterojunction Tandem Solar Cells with Nanocrystalline Si/SiO x Tunnel Junction

Author

Listed:
  • Lucia V. Mercaldo

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Eugenia Bobeico

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Antonella De Maria

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Marco Della Noce

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Manuela Ferrara

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Vera La Ferrara

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Laura Lancellotti

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Gabriella Rametta

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Gennaro V. Sannino

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy
    Department of Chemical Sciences, Monte Sant’Angelo Campus, University of Naples Federico II, Via Cinthia 21, 80126 Naples, Italy)

  • Iurie Usatii

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

  • Paola Delli Veneri

    (Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA), Portici Research Center, Piazzale E. Fermi, 80055 Portici, Italy)

Abstract

Perovskite/silicon tandem solar cells have strong potential for high efficiency and low cost photovoltaics. In monolithic (two-terminal) configurations, one key element is the interconnection region of the two subcells, which should be designed for optimal light management and prevention of parasitic p/n junctions. We investigated monolithic perovskite/silicon-heterojunction (SHJ) tandem solar cells with a p/n nanocrystalline silicon/silicon-oxide recombination junction for improved infrared light management. This design can additionally provide for resilience to shunts and simplified cell processing. We probed modified SHJ solar cells, made from double-side polished n-type Si wafers, which included the proposed front-side p/n tunnel junction with the p-type film simultaneously functioning as selective charge transport layer for the SHJ bottom cell, trying different thicknesses for the n-type layer. Full tandem devices were then tested, by applying a planar n-i-p mixed-cation mixed-halide perovskite top cell, fabricated via low temperature solution methods to be compatible with the processed Si wafer. We demonstrate the feasibility of this tandem cell configuration over a 1 cm 2 area with negligible J-V hysteresis and a V OC ~1.8 V, matching the sum of the V OC -s contributed by the two components.

Suggested Citation

  • Lucia V. Mercaldo & Eugenia Bobeico & Antonella De Maria & Marco Della Noce & Manuela Ferrara & Vera La Ferrara & Laura Lancellotti & Gabriella Rametta & Gennaro V. Sannino & Iurie Usatii & Paola Dell, 2021. "Monolithic Perovskite/Silicon-Heterojunction Tandem Solar Cells with Nanocrystalline Si/SiO x Tunnel Junction," Energies, MDPI, vol. 14(22), pages 1-13, November.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:22:p:7684-:d:680891
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    References listed on IDEAS

    as
    1. Lucia V. Mercaldo & Iurie Usatii & Paola Delli Veneri, 2016. "Advances in Thin-Film Si Solar Cells by Means of SiO x Alloys," Energies, MDPI, vol. 9(3), pages 1-13, March.
    2. Jaeki Jeong & Minjin Kim & Jongdeuk Seo & Haizhou Lu & Paramvir Ahlawat & Aditya Mishra & Yingguo Yang & Michael A. Hope & Felix T. Eickemeyer & Maengsuk Kim & Yung Jin Yoon & In Woo Choi & Barbara Pr, 2021. "Pseudo-halide anion engineering for α-FAPbI3 perovskite solar cells," Nature, Nature, vol. 592(7854), pages 381-385, April.
    3. Kunta Yoshikawa & Hayato Kawasaki & Wataru Yoshida & Toru Irie & Katsunori Konishi & Kunihiro Nakano & Toshihiko Uto & Daisuke Adachi & Masanori Kanematsu & Hisashi Uzu & Kenji Yamamoto, 2017. "Silicon heterojunction solar cell with interdigitated back contacts for a photoconversion efficiency over 26%," Nature Energy, Nature, vol. 2(5), pages 1-8, May.
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    Cited by:

    1. Jianqin Li & Feng Wen & Shenghao Wang, 2023. "Perovskite Tandem Solar Cell Technologies," Energies, MDPI, vol. 16(4), pages 1-3, February.

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