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CO 2 and CH 4 Adsorption Behavior of Biomass-Based Activated Carbons

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  • Deneb Peredo-Mancilla

    (CNRS/Total/Univ Pau & Pays Adour/ E2S UPPA, Laboratoire des Fluides Complexes et Leurs Reservoirs-IPRA, UMRS5150, 64000 Pau, France
    Univ Pau & Pays Adour/ E2S UPPA, Laboratoire de Thermique, Energetique et Procedes-IPRA, EA1932, 64000 Pau, France)

  • Imen Ghouma

    (Institut de Sciences des Matériaux de Mulhouse, UMR 7661 CNRS, 15 rue Jean Starcky, 68057 Mulhouse, France)

  • Cecile Hort

    (Univ Pau & Pays Adour/ E2S UPPA, Laboratoire de Thermique, Energetique et Procedes-IPRA, EA1932, 64000 Pau, France)

  • Camelia Matei Ghimbeu

    (Institut de Sciences des Matériaux de Mulhouse, UMR 7661 CNRS, 15 rue Jean Starcky, 68057 Mulhouse, France)

  • Mejdi Jeguirim

    (Institut de Sciences des Matériaux de Mulhouse, UMR 7661 CNRS, 15 rue Jean Starcky, 68057 Mulhouse, France)

  • David Bessieres

    (CNRS/Total/Univ Pau & Pays Adour/ E2S UPPA, Laboratoire des Fluides Complexes et Leurs Reservoirs-IPRA, UMRS5150, 64000 Pau, France)

Abstract

The aim of the present work is to study the effect of different activation methods for the production of a biomass-based activated carbon on the CO 2 and CH 4 adsorption. The influence of the activation method on the adsorption uptake was studied using three activated carbons obtained by different activation methods (H 3 PO 4 chemical activation and H 2 O and CO 2 physical activation) of olive stones. Methane and carbon dioxide pure gas adsorption experiments were carried out at two working temperatures (303.15 and 323.15 K). The influence of the activation method on the adsorption uptake was studied in terms of both textural properties and surface chemistry. For the three adsorbents, the CO 2 adsorption was more important than that of CH 4 . The chemically-activated carbon presented a higher specific surface area and micropore volume, which led to a higher adsorption capacity of both CO 2 and CH 4 . For methane adsorption, the presence of mesopores facilitated the diffusion of the gas molecules into the micropores. In the case of carbon dioxide adsorption, the presence of more oxygen groups on the water vapor-activated carbon enhanced its adsorption capacity.

Suggested Citation

  • Deneb Peredo-Mancilla & Imen Ghouma & Cecile Hort & Camelia Matei Ghimbeu & Mejdi Jeguirim & David Bessieres, 2018. "CO 2 and CH 4 Adsorption Behavior of Biomass-Based Activated Carbons," Energies, MDPI, vol. 11(11), pages 1-13, November.
    • Handle: RePEc:gam:jeners:v:11:y:2018:i:11:p:3136-:d:182400
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    References listed on IDEAS

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    1. Imen Ghouma & Mejdi Jeguirim & Uta Sager & Lionel Limousy & Simona Bennici & Eckhard Däuber & Christof Asbach & Roman Ligotski & Frank Schmidt & Abdelmottaleb Ouederni, 2017. "The Potential of Activated Carbon Made of Agro-Industrial Residues in NO x Immissions Abatement," Energies, MDPI, vol. 10(10), pages 1-15, September.
    2. Silvia Román & Beatriz Ledesma & Andrés Álvarez-Murillo & Awf Al-Kassir & Talal Yusaf, 2017. "Dependence of the Microporosity of Activated Carbons on the Lignocellulosic Composition of the Precursors," Energies, MDPI, vol. 10(4), pages 1-11, April.
    3. Hao, Wenming & Björkman, Eva & Lilliestråle, Malte & Hedin, Niklas, 2013. "Activated carbons prepared from hydrothermally carbonized waste biomass used as adsorbents for CO2," Applied Energy, Elsevier, vol. 112(C), pages 526-532.
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    1. Mudassir, Muhammad Ahmad & Kousar, Shazia & Ehsan, Muhammad & Usama, Muhammad & Sattar, Umer & Aleem, Muhammad & Naheed, Irum & Saeed, Osama Bin & Ahmad, Mehmood & Akbar, Hafiz Favad & Ud Din, Muhamma, 2023. "Emulsion-derived porous carbon-based materials for energy and environmental applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 185(C).

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    Keywords

    CO2 adsorption; CH4 adsorption; biomass; activated carbon;
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