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CO2 adsorbent pellets produced from pine sawdust: Effect of coal tar pitch addition

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  • Plaza, M.G.
  • Durán, I.
  • Rubiera, F.
  • Pevida, C.

Abstract

The main drawbacks of developing carbon adsorbents from pine sawdust, an abundant biomass feedstock, are the low carbon yield of the process and the poor mechanical properties of the resulting carbons. In an attempt to overcome these limitations, the effect of the addition of coal tar pitch was assessed. Adsorbent pellets were produced from pine sawdust and coal tar pitch by activation with CO2. The preparation process was optimized by using as decision variables the carbon yield and the adsorption performance of the adsorbents in conditions representative of post-combustion capture applications (10% CO2 at atmospheric pressure and at 50°C). Subjecting the composite pellets to a pre-oxidation treatment with air increased the carbon yield of the production process, and also improved the adsorption kinetics and capacity of the final adsorbents. The prepared adsorbents present a high carbon yield, a superior mechanical resistance and a competitive adsorption performance.

Suggested Citation

  • Plaza, M.G. & Durán, I. & Rubiera, F. & Pevida, C., 2015. "CO2 adsorbent pellets produced from pine sawdust: Effect of coal tar pitch addition," Applied Energy, Elsevier, vol. 144(C), pages 182-192.
    • Handle: RePEc:eee:appene:v:144:y:2015:i:c:p:182-192
    DOI: 10.1016/j.apenergy.2014.12.090
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    References listed on IDEAS

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    Cited by:

    1. Marcin Bielecki & Valentina Zubkova & Andrzej Strojwas, 2023. "An Analysis of the Influence of Low Density Polyethylene, Novolac, and Coal Tar Pitch Additives on the Decrease in Content of Impurities Emitted from Densified Pea Husks during the Process of Their Py," Energies, MDPI, vol. 16(6), pages 1-16, March.
    2. Nausika Querejeta & M. Victoria Gil & Fernando Rubiera & Covadonga Pevida, 2018. "Sustainable coffee†based CO2 adsorbents: toward a greener production via hydrothermal carbonization," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 8(2), pages 309-323, April.
    3. Junya Wang & Qiuyun Pu & Ping Ning & Shijian Lu, 2021. "Activated carbon‐based composites for capturing CO2: a review," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(2), pages 377-393, April.
    4. Inés Durán & Fernando Rubiera & Covadonga Pevida, 2017. "Separation of CO 2 in a Solid Waste Management Incineration Facility Using Activated Carbon Derived from Pine Sawdust," Energies, MDPI, vol. 10(6), pages 1-20, June.
    5. Jia Yen Lai & Lock Hei Ngu & Siti Salwa Hashim, 2021. "A review of CO2 adsorbents performance for different carbon capture technology processes conditions," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(5), pages 1076-1117, October.

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    Keywords

    Biomass; Adsorbents; Carbon; CO2 capture;
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