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Recent advances in supercritical water gasification of biowaste catalyzed by transition metal-based catalysts for hydrogen production

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  • Su, Hongcai
  • Yan, Mi
  • Wang, Shurong

Abstract

Supercritical water gasification (SCWG) is a remarkably efficient technology for converting wet biowaste (such as food waste, paper industrial waste, sewage sludge, agricultural waste, and forestry residue) into energy in the form of hydrogen-rich syngas. Catalysts have been widely used for promoting the hydrogen production rate of SCWG at mild reaction temperatures. In this regard, transition metal-based catalysts have attracted extensive attention from researchers due to their excellent performance and recyclability. Herein, the catalytic effects of transition metal-based catalysts on the SCWG of biowaste are reviewed, including the influence of active components, synthetic methods, and support materials. The modification of transition metal-based catalysts (rare earth oxide-promoted catalysts, noble-metal bimetallic catalysts, noble-metal-free bimetallic catalysts, and alkaline-earth metal-promoted catalysts) is also discussed. Finally, technical challenges and future perspectives for the development of transition metal-based catalysts in the SCWG of biowaste are presented. This review paper aims at providing an important reference for the design of transition metal-based catalysts with excellent catalytic performance and physicochemical properties and their applications in the SCWG of biowaste.

Suggested Citation

  • Su, Hongcai & Yan, Mi & Wang, Shurong, 2022. "Recent advances in supercritical water gasification of biowaste catalyzed by transition metal-based catalysts for hydrogen production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 154(C).
    • Handle: RePEc:eee:rensus:v:154:y:2022:i:c:s1364032121010984
    DOI: 10.1016/j.rser.2021.111831
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