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Supercritical water gasification of biomass model compounds: A review

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  • Hu, Yulin
  • Gong, Mengyue
  • Xing, Xuelian
  • Wang, Haoyu
  • Zeng, Yimin
  • Xu, Chunbao Charles

Abstract

In recent decades, conversion of bio-renewable resources to biofuels or bio-based chemicals has received a great deal of attention, owing to the resource exhaustion, environmental concerns, and socio-economic issues of fossil fuels. One of the promising biomass conversion routes is the supercritical water gasification (SCWG) of biomass for producing H2 or combustible gases. SCWG is an effective conversion technology, particularly for high water-containing feedstocks, because of its unique advantage by avoiding the costly feedstock de-watering/drying process. To improve gasification performance, it is necessary to have a deeper understanding of the basic chemistry and kinetics of biomass SCWG. Therefore, this review focuses on the performance (chemistry and kinetics) of SCWG of biomass model compounds (cellulose, hemicellulose, lignin, lipid, and protein), and more importantly the binary or multi-component systems to elucidate the interaction effects induced by two or more biomass components in supercritical water (SCW). In addition, the advantages and technical challenges for using SCW as the reaction medium are discussed. Finally, the future R&D directions are presented.

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  • Hu, Yulin & Gong, Mengyue & Xing, Xuelian & Wang, Haoyu & Zeng, Yimin & Xu, Chunbao Charles, 2020. "Supercritical water gasification of biomass model compounds: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 118(C).
    • Handle: RePEc:eee:rensus:v:118:y:2020:i:c:s1364032119307373
    DOI: 10.1016/j.rser.2019.109529
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    3. Kapil Khandelwal & Philip Boahene & Sonil Nanda & Ajay K. Dalai, 2023. "Hydrogen Production from Supercritical Water Gasification of Model Compounds of Crude Glycerol from Biodiesel Industries," Energies, MDPI, vol. 16(9), pages 1-19, April.
    4. Radhakrishnan, Rokesh & Patra, Pradipta & Das, Manali & Ghosh, Amit, 2021. "Recent advancements in the ionic liquid mediated lignin valorization for the production of renewable materials and value-added chemicals," Renewable and Sustainable Energy Reviews, Elsevier, vol. 149(C).
    5. Li, Kaiyang & Zeng, Yimin, 2022. "Corrosion of heat exchanger materials in co-combustion thermal power plants," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    6. Fózer, Dániel & Volanti, Mirco & Passarini, Fabrizio & Varbanov, Petar Sabev & Klemeš, Jiří Jaromír & Mizsey, Péter, 2020. "Bioenergy with carbon emissions capture and utilisation towards GHG neutrality: Power-to-Gas storage via hydrothermal gasification," Applied Energy, Elsevier, vol. 280(C).
    7. Chen, Yunan & Yi, Lei & Yin, Jiarong & Jin, Hui & Guo, Liejin, 2022. "Sewage sludge gasification in supercritical water with fluidized bed reactor: Reaction and product characteristics," Energy, Elsevier, vol. 239(PB).
    8. Ramin Azargohar & Sonil Nanda & He Cheng & Ajay K. Dalai, 2022. "Potential Application of Canola Hull Fuel Pellets for the Production of Synthesis Gas and Hydrogen," Energies, MDPI, vol. 15(22), pages 1-15, November.

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