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Model prediction of effects of operating parameters on proton exchange membrane fuel cell performance

Author

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  • Yuan, Wei
  • Tang, Yong
  • Pan, Minqiang
  • Li, Zongtao
  • Tang, Biao

Abstract

The performance of a proton exchange membrane (PEM) fuel cell is greatly affected by the operating parameters. Appropriate operating parameters are necessary for PEM fuel cells to maintain stable performance. A three-dimensional multi-phase fuel cell model (FCM) is developed to predict the effects of operating parameters (e.g. operating pressure, fuel cell temperature, relative humidity of reactant gases, and air stoichiometric ratio) on the performance of PEM fuel cells. The model presented in this paper is a typical nine-layer FCM that consists of current collectors, flow channels, gas diffusion layers, catalysts layers at the anode and the cathode as well as the membrane. A commercial Computational Fluid Dynamics (CFD) software package Fluent is used to solve this predictive model through SIMPLE algorithm and the modeling results are illustrated via polarization curves including I–V and I–P curves. The results indicate that the cell performance can be enhanced by increasing operating pressure and operating temperature. The anode humidification has more significant influences on the cell performance than the cathode humidification, and the best performance occurs at moderate air relative humidity while the hydrogen is fully humidified. In addition, the cell performance proves to be improved with the increase of air stoichiometric ratio. Based on these conclusions, several suggestions for engineering practice are also provided.

Suggested Citation

  • Yuan, Wei & Tang, Yong & Pan, Minqiang & Li, Zongtao & Tang, Biao, 2010. "Model prediction of effects of operating parameters on proton exchange membrane fuel cell performance," Renewable Energy, Elsevier, vol. 35(3), pages 656-666.
    • Handle: RePEc:eee:renene:v:35:y:2010:i:3:p:656-666
    DOI: 10.1016/j.renene.2009.08.017
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    References listed on IDEAS

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    1. Yu, Sangseok & Jung, Dohoy, 2008. "Thermal management strategy for a proton exchange membrane fuel cell system with a large active cell area," Renewable Energy, Elsevier, vol. 33(12), pages 2540-2548.
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    2. Zhang, Jian & Huang, Pengyi & Ding, Honghui & Xin, Dongqun & Sun, Shufeng, 2023. "Investigation of the three-dimensional flow field for proton exchange membrane fuel cell with additive manufactured stainless steel bipolar plates: Numerical simulation and experiments," Energy, Elsevier, vol. 269(C).
    3. Lakshminarayana, G. & Nogami, Masayuki & Kityk, I.V., 2010. "Synthesis and characterization of anhydrous proton conducting inorganic–organic composite membranes for medium temperature proton exchange membrane fuel cells (PEMFCs)," Energy, Elsevier, vol. 35(12), pages 5260-5268.
    4. Wang, Zhenhao & Hu, Kaihua & Zhang, Jian & Ding, Honghui & Xin, Dongqun & Zhang, Fengyun & Sun, Shufeng, 2023. "Gas-liquid mass transfer characteristics of a novel three-dimensional flow field bipolar plate for laser additive manufacturing of proton exchange membrane fuel cell," Renewable Energy, Elsevier, vol. 212(C), pages 308-319.
    5. González-Espasandín, Óscar & Leo, Teresa J. & Raso, Miguel A. & Navarro, Emilio, 2019. "Direct methanol fuel cell (DMFC) and H2 proton exchange membrane fuel (PEMFC/H2) cell performance under atmospheric flight conditions of Unmanned Aerial Vehicles," Renewable Energy, Elsevier, vol. 130(C), pages 762-773.
    6. Jiang, Ke & Zhao, Taotao & Fan, Wenxuan & Liu, Zhenning & Lu, Guolong, 2023. "Ramped step flow field to enhance mass transfer capacity and performance for PEMFC," Renewable Energy, Elsevier, vol. 219(P2).
    7. Asadi, Mohammad Reza & Ghasabehi, Mehrdad & Ghanbari, Sina & Shams, Mehrzad, 2024. "The optimization of an innovative interdigitated flow field proton exchange membrane fuel cell by using artificial intelligence," Energy, Elsevier, vol. 290(C).
    8. Movahedi, M. & Ramiar, A. & Ranjber, A.A., 2018. "3D numerical investigation of clamping pressure effect on the performance of proton exchange membrane fuel cell with interdigitated flow field," Energy, Elsevier, vol. 142(C), pages 617-632.
    9. Chen Li & Ashanti M. Sallee & Xiaoyu Zhang & Sandeep Kumar, 2018. "Electrochemical Hydrogenation of Acetone to Produce Isopropanol Using a Polymer Electrolyte Membrane Reactor," Energies, MDPI, vol. 11(10), pages 1-17, October.
    10. Tzelepis, Stefanos & Kavadias, Kosmas A. & Marnellos, George E. & Xydis, George, 2021. "A review study on proton exchange membrane fuel cell electrochemical performance focusing on anode and cathode catalyst layer modelling at macroscopic level," Renewable and Sustainable Energy Reviews, Elsevier, vol. 151(C).
    11. Feng, Pengfei & Tan, Ligang & Cao, Yucheng & Chen, Ding, 2023. "Numerical investigations of two-phase flow coupled with species transport in proton exchange membrane fuel cells," Energy, Elsevier, vol. 278(PA).
    12. Jian, Qi-fei & Ma, Guang-qing & Qiu, Xiao-liang, 2014. "Influences of gas relative humidity on the temperature of membrane in PEMFC with interdigitated flow field," Renewable Energy, Elsevier, vol. 62(C), pages 129-136.
    13. Wu, Ziyao & Pei, Pucheng & Xu, Huachi & Jia, Xiaoning & Ren, Peng & Wang, Bozheng, 2019. "Study on the effect of membrane electrode assembly parameters on polymer electrolyte membrane fuel cell performance by galvanostatic charging method," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    14. Zheng Huang & Laisuo Su & Yunjie Yang & Linsong Gao & Xinyu Liu & Heng Huang & Yubai Li & Yongchen Song, 2023. "Three-Dimensional Simulation on the Effects of Different Parameters and Pt Loading on the Long-Term Performance of Proton Exchange Membrane Fuel Cells," Sustainability, MDPI, vol. 15(4), pages 1-22, February.
    15. Abdollahipour, Armin & Sayyaadi, Hoseyn, 2022. "A novel electrochemical refrigeration system based on the combined proton exchange membrane fuel cell-electrolyzer," Applied Energy, Elsevier, vol. 316(C).
    16. Deng, Hao & Wang, Dawei & Xie, Xu & Zhou, Yibo & Yin, Yan & Du, Qing & Jiao, Kui, 2016. "Modeling of hydrogen alkaline membrane fuel cell with interfacial effect and water management optimization," Renewable Energy, Elsevier, vol. 91(C), pages 166-177.
    17. Gong, Fan & Yang, Xiaolong & Zhang, Xun & Mao, Zongqiang & Gao, Weitao & Wang, Cheng, 2023. "The study of Tesla valve flow field on the net power of proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 329(C).
    18. Abdollahipour, Armin & Sayyaadi, Hoseyn, 2022. "Optimal design of a hybrid power generation system based on integrating PEM fuel cell and PEM electrolyzer as a moderator for micro-renewable energy systems," Energy, Elsevier, vol. 260(C).
    19. Melika Hinaje & Stéphane Raël & Panee Noiying & Dinh An Nguyen & Bernard Davat, 2012. "An Equivalent Electrical Circuit Model of Proton Exchange Membrane Fuel Cells Based on Mathematical Modelling," Energies, MDPI, vol. 5(8), pages 1-21, July.
    20. Li, Wenkai & Zhang, Qinglei & Wang, Chao & Yan, Xiaohui & Shen, Shuiyun & Xia, Guofeng & Zhu, Fengjuan & Zhang, Junliang, 2017. "Experimental and numerical analysis of a three-dimensional flow field for PEMFCs," Applied Energy, Elsevier, vol. 195(C), pages 278-288.
    21. Ahmed G. Abokhalil & Mohammad Alobaid & Ahmed Al Makky, 2023. "Innovative Approaches to Enhance the Performance and Durability of Proton Exchange Membrane Fuel Cells," Energies, MDPI, vol. 16(14), pages 1-13, July.

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